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Reversible Three-Color Fluorescence Switching of an Organic Molecule in the Solid State via "PumpTrigger" Optical Manipulation¥R. Yang, X. Ren, L. Mei, G. Pan, X.-Z. Li, Z. Wu, S. Zhang, W. Ma, W. Yu, H.-H. Fang, C. Li, M.-Q. Zhu, Z. Hu, T. Sun, B. Xu and W. Tian¥2022¥Angewandte Chemie - International Edition¥14337851¥61¥20¥In photoswitches that undergo fluorescence switching upon ultraviolet irradiation, photoluminescence and photoisomerization often occur simultaneously, leading to unstable fluorescence properties. Here, we successfully demonstrated reversible solid-state triple fluorescence switching through "PumpTrigger" multiphoton manipulation. A novel fluorescence photoswitch, BOSA-SP, achieved green, yellow, and red fluorescence under excitation by pump light and isomerization induced by trigger light. The energy ranges of photoexcitation and photoisomerization did not overlap, enabling appropriate selection of the multiphoton light for "pump" and "trigger" photoswitching, respectively. Additionally, the large free volume of the spiropyran (SP) moiety in the solid state promoted reversible photoisomerization. Switching between "pump" and "trigger" light is useful for three-color tunable switching cell imaging, which can be exploited in programmable fluorescence switching. Furthermore, we exploited reversible dual-fluorescence switching in a single molecular system to successfully achieve two-color super-resolution imaging. 2022 Wiley-VCH GmbH.¥internal-pdf://0789088499/Reversible Three-Color Fluorescence Switching.pdf¥10.1002/anie.202117158¥https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/anie.202117158?download=true¥sci&ei
期刊论文
Angewandte Chemie - International Edition, 2022, 卷号: 61, 期号: 20
作者:
R. Yang
;
X. Ren
;
L. Mei
;
G. Pan
;
X.-Z. Li
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  |  
浏览/下载:10/0
  |  
提交时间:2023/06/14
Reversible Three-Color Fluorescence Switching of an Organic Molecule in the Solid State via "PumpTrigger" Optical Manipulation
期刊论文
Angewandte Chemie - International Edition, 2022, 卷号: 61, 期号: 20
作者:
R. Yang
;
X. Ren
;
L. Mei
;
G. Pan
;
X.-Z. Li
收藏
  |  
浏览/下载:6/0
  |  
提交时间:2023/07/17
Simulation analysis and comparison of the effects of aberrations on multiphoton fluorescent light sheets
期刊论文
Optics Communications, 2021, 卷号: 482
作者:
W. Sun
;
N. Li
;
C. Zhang
;
Q. Mu
;
X. Zhang
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浏览/下载:4/0
  |  
提交时间:2022/06/13
Wavelength-dependent nonsequential double ionization of magnesium by intense femtosecond laser pulses
期刊论文
PHYSICAL REVIEW A, 2019, 卷号: 100, 期号: 3, 页码: 6
作者:
Kang, HuiPeng
;
Chen, Shi
;
Wang, YanLan
;
Chu, Wei
;
Yao, JinPing
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浏览/下载:57/0
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提交时间:2019/12/06
Striking Isotopologue-Dependent Photodissociation Dynamics of Water Molecules: The Signature of an Accidental Resonance
期刊论文
JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2019, 卷号: 10, 期号: 15, 页码: 4209-4214
作者:
Chang, Yao
;
Chen, Zhichao
;
Zhou, Jiami
;
Luo, Zijie
;
He, Zhigan
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  |  
浏览/下载:53/0
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提交时间:2019/12/02
Efficient Red/Near-Infrared-Emissive Carbon Nanodots with Multiphoton Excited Upconversion Fluorescence
期刊论文
ADVANCED SCIENCE, 2019, 页码: 10
作者:
Liu, Kai-Kai
;
Song, Shi-Yu
;
Sui, Lai-Zhi
;
Wu, Si-Xuan
;
Jing, Peng-Tao
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  |  
浏览/下载:198/0
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提交时间:2019/12/02
carbon nanodots
cellular imaging
fluorescence
multiphoton excitation
red/near-infrared
Integrating temporal and spatial control of electronic transitions for bright multiphoton upconversion
期刊论文
NATURE COMMUNICATIONS, 2019, 卷号: 10
作者:
Sun, Tianying
;
Li, Yuhua
;
Ho, Wai Lok
;
Zhu, Qi
;
Chen, Xian
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  |  
浏览/下载:52/0
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提交时间:2019/05/15
Branching Ratios of the N(D-2(3/2)0) and N(D-2(5/2)0) Spin-Orbit States Produced in the State-Selected Photodissociation of N-2 Determined Using Time-Sliced Velocity-Mapped-Imaging Photoionization Mass Spectrometry (TS-VMI-PI-MS)
期刊论文
JOURNAL OF PHYSICAL CHEMISTRY A, 2019, 卷号: 123, 期号: 12, 页码: 2289-2300
作者:
Jackson, William M.
;
Ng, Cheuk-Yiu
;
Kalogerakis, Konstantinos S.
;
Liu, Kai
;
Chang, Yih Chung
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浏览/下载:53/0
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提交时间:2019/06/24
Photobleaching of ultrashort pulses with different repetition rates in two-photon excitation microscopy
期刊论文
LASER PHYSICS, 2019, 卷号: 29
作者:
Niu, Fuzeng
;
Wu, Runlong
;
Wu, Danlei
;
Gou, Dongzhou
;
Feng, Lishuang
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浏览/下载:10/0
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提交时间:2019/12/30
ultrafast lasers
nonlinear optics
multiphoton processes
fluorescence microscopy
Thermally Activated Upconversion Near-Infrared Photoluminescence from Carbon Dots Synthesized via Microwave Assisted Exfoliation
期刊论文
Small, 2019, 卷号: 15, 期号: 50, 页码: 7
作者:
D.Li
;
C.Liang
;
E.V.Ushakova
;
M.H.Sun
;
X.D.Huang
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浏览/下载:0/0
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提交时间:2020/08/24
carbon dots,exfoliation,near-infrared absorption,near-infrared,photoluminescence,upconversion photoluminescence,graphene quantum dots,fluorescence
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