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Modulating Charge Transport from Thermally Activated to "Band-Like" Through Interfacial Bottom-Up Binding Capability of Bilayer Polymer Dielectrics¥Y. Zheng, H. Lin, T. Jiang, D. Zhu, S. Qi, W. Li, L. Li, D. Ji and W. Hu¥2022¥1616301X¥The disordered chain arrangement of polymer dielectrics has complex both internal and external effects on system performance, which generally stimulates the weak acquisition and grain boundaries of vapor-deposited organic small molecule films (VDOSMFs) with thermally activated charge transport. As a result, achieving "band-like" transmission of VDOSMs on polymer dielectrics is attempting to prove to be a major challenge. Three types of bi-polymer dielectrics are developed to modulate charge transport from thermally activated mode to "band-like" transport at the interfacial level. The bottom consisting of a polyimide layer is critical to interfacial modulation, which shows the selectively binding capability with up-dielectric layers to realize the modulation of charge transport, as corroborated by interface characterization and density functional-based tight-binding calculation. The findings provide an effective strategy for modulating the charge transport through polymer dielectric engineering and also recommend a podium to further comprehend the electrical characteristics of small molecules in organic thin-film transistors. 2022 Wiley-VCH GmbH.¥internal-pdf://1153944661/Modulating Charge Transport from Thermally Act.pdf¥10.1002/adfm.202211742¥https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202211742?download=true¥ei
期刊论文
1616301X, 2022
作者:
Y. Zheng
;
H. Lin
;
T. Jiang
;
D. Zhu
;
S. Qi
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  |  
浏览/下载:1/0
  |  
提交时间:2023/06/14
Modulating Charge Transport from Thermally Activated to "Band-Like" Through Interfacial Bottom-Up Binding Capability of Bilayer Polymer Dielectrics
期刊论文
1616301X, 2022
作者:
Y. Zheng
;
H. Lin
;
T. Jiang
;
D. Zhu
;
S. Qi
收藏
  |  
浏览/下载:1/0
  |  
提交时间:2023/07/17
Naphthalene diimide based near-infrared luminogens with aggregation-induced emission characteristics for biological imaging and high mobility ambipolar transistors
期刊论文
SCIENCE CHINA-CHEMISTRY, 2020, 页码: 10
作者:
Guo, De
;
Li, Lin
;
Zhu, Xianqi
;
Heeney, Martin
;
Li, Jing
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  |  
浏览/下载:21/0
  |  
提交时间:2020/08/24
aggregation induced emission (AIE)
naphthalene diimides (NDI)
near-infrared (NIR) solid emission
organic field effect transistors (OFETs)
bio-imaging
Self-assembly crystal microribbons with nucleation additive for high-performance organic thin film transistors
期刊论文
JAPANESE JOURNAL OF APPLIED PHYSICS, 2019, 卷号: 58
作者:
He, Zhengran
;
Asare-Yeboah, Kyeiwaa
;
Zhang, Ziyang
;
Bi, Sheng
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浏览/下载:16/0
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提交时间:2019/12/02
Poly(alpha-methylstyrene) polymer and small-molecule semiconductor blend with reduced crystal misorientation for organic thin film transistors
期刊论文
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2019, 卷号: 30, 页码: 14335-14343
作者:
He, Zhengran
;
Zhang, Ziyang
;
Asare-Yeboah, Kyeiwaa
;
Bi, Sheng
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浏览/下载:23/0
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提交时间:2019/12/02
High-Performance Organic-Inorganic Hybrid Thin-Film Transistors with Interesting Synaptic Behaviors
期刊论文
PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE, 2019, 卷号: 216
作者:
Zhu, Huichao
;
Mu, Hongjian
;
Cai, Zhaoyun
;
Chu, Xuefeng
;
Yang, Xiaotian
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浏览/下载:27/0
  |  
提交时间:2019/12/02
artificial synapses
electrochromism
electrolyte-gated transistors
organic-inorganic hybrid electrolytes
tungsten oxides
Long-range crystal alignment with polymer additive for organic thin film transistors
期刊论文
JOURNAL OF POLYMER RESEARCH, 2019, 卷号: 26
作者:
He, Zhengran
;
Zhang, Ziyang
;
Bi, Sheng
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浏览/下载:2/0
  |  
提交时间:2019/12/02
Crystallization
Charge transport
Small-molecule semiconductor
Polymer additive
Organic thin film transistors
Direct Arylation Polycondensation Synthesis of High Mobility Conjugated Polymers
期刊论文
ACTA POLYMERICA SINICA, 2019, 卷号: Vol.50 No.2, 页码: 109-117
作者:
Geng, Y.-H.
;
Sui, Y.
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浏览/下载:7/0
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提交时间:2019/11/21
Direct arylation polycondensation
Conjugated polymers
Semiconducting materials
Organic thin-film transistors
Charge carrier mobility
Design strategies of n-type conjugated polymers for organic thin-film transistors
期刊论文
Materials Chemistry Frontiers, 2019, 卷号: Vol.3 No.10, 页码: 1932-1951
作者:
Sui, Y.a
;
Deng, Y.a
;
Du, T.a
;
Shi, Y.a
;
Geng, Y.a,b
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浏览/下载:12/0
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提交时间:2019/11/26
High performance n-type vertical organic phototransistors
期刊论文
ORGANIC ELECTRONICS, 2019, 卷号: 67, 页码: 200-207
作者:
Yeliu, Kaiheng
;
Zhong, Jianfeng
;
Wang, Xiumei
;
Yan, Yujie
;
Chen, Qizhen
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  |  
浏览/下载:19/0
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提交时间:2019/11/21
n-type organic semiconductor
Organic phototransistors
Organic thin-film transistors
Vertical structure
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