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Modulating Charge Transport from Thermally Activated to "Band-Like" Through Interfacial Bottom-Up Binding Capability of Bilayer Polymer Dielectrics¥Y. Zheng, H. Lin, T. Jiang, D. Zhu, S. Qi, W. Li, L. Li, D. Ji and W. Hu¥2022¥1616301X¥The disordered chain arrangement of polymer dielectrics has complex both internal and external effects on system performance, which generally stimulates the weak acquisition and grain boundaries of vapor-deposited organic small molecule films (VDOSMFs) with thermally activated charge transport. As a result, achieving "band-like" transmission of VDOSMs on polymer dielectrics is attempting to prove to be a major challenge. Three types of bi-polymer dielectrics are developed to modulate charge transport from thermally activated mode to "band-like" transport at the interfacial level. The bottom consisting of a polyimide layer is critical to interfacial modulation, which shows the selectively binding capability with up-dielectric layers to realize the modulation of charge transport, as corroborated by interface characterization and density functional-based tight-binding calculation. The findings provide an effective strategy for modulating the charge transport through polymer dielectric engineering and also recommend a podium to further comprehend the electrical characteristics of small molecules in organic thin-film transistors. 2022 Wiley-VCH GmbH.¥internal-pdf://1153944661/Modulating Charge Transport from Thermally Act.pdf¥10.1002/adfm.202211742¥https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202211742?download=true¥ei
期刊论文
1616301X, 2022
作者:
Y. Zheng
;
H. Lin
;
T. Jiang
;
D. Zhu
;
S. Qi
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浏览/下载:1/0
  |  
提交时间:2023/06/14
Modulating Charge Transport from Thermally Activated to "Band-Like" Through Interfacial Bottom-Up Binding Capability of Bilayer Polymer Dielectrics
期刊论文
1616301X, 2022
作者:
Y. Zheng
;
H. Lin
;
T. Jiang
;
D. Zhu
;
S. Qi
收藏
  |  
浏览/下载:1/0
  |  
提交时间:2023/07/17
A simple strategy to prepare functional PI microspheres by constructing coating on PAA microspheres followed thermal imidization reaction
期刊论文
COMPOSITES COMMUNICATIONS, 2021, 卷号: 24
作者:
Zhang, Qian
;
Han, Yazhe
;
Ding, Xin
;
Zhang, Ping
;
Wang, Yanyan
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浏览/下载:43/0
  |  
提交时间:2021/05/06
Polyimide
Microspheres
Phase separation
Composite material
Imidization-induced carbon nitride nanosheets orientation towards highly thermally conductive polyimide film with superior flexibility and electrical insulation
期刊论文
COMPOSITES PART B-ENGINEERING, 2020, 卷号: 199
作者:
Wang, Yanyan
;
Zhang, Xian
;
Ding, Xin
;
Zhang, Ping
;
Shu, Mengting
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浏览/下载:65/0
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提交时间:2020/11/30
Carbon nitride nanosheets
Nanocomposite film
Thermal conductivity
Electrical insulation
Mechanical flexibility
Thermally rearranged polymer membranes containing highly rigid biphenyl ortho-hydroxyl diamine for hydrogen separation
期刊论文
JOURNAL OF MEMBRANE SCIENCE, 2020, 卷号: 604, 页码: 12
作者:
Hu, Xiaofan
;
Lee, Won Hee
;
Zhao, Jiayi
;
Kim, Ju Sung
;
Wang, Zhen
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浏览/下载:17/0
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提交时间:2020/09/22
Polyimides
TR polymers
High rigidity
Hydrogen separation
Membranes
Modeling Gas and Vapor Sorption and Swelling in Triptycene-Based Polybenzoxazole: Evidence for Entropy-Driven Sorption Behavior
期刊论文
MACROMOLECULES, 2019, 卷号: 52, 期号: 11, 页码: 4385-4395
作者:
Loianno, Valerio
;
Zhang, Qinnan
;
Luo, Shuangjiang
;
Guo, Ruilan
;
Galizia, Michele
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浏览/下载:44/0
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提交时间:2019/09/03
Polarization-induced alignment of azobenzene/fluorinated polyimide for three-dimensional shape-persistent and photo-responsive elastic helixes
期刊论文
Composites Science and Technology, 2019, 卷号: Vol.169, 页码: 158-166
作者:
Li, S.
;
Feng, Y.
;
Wang, W.
;
Ji, T.
;
Han, J.
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浏览/下载:9/0
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提交时间:2019/11/21
Azobenzene-polyimide
Elasticity
Helix
Photoresponse
Shape-persistence
Synthesis and Properties of High Performance Functional Polyimides Containing Rigid Nonplanar Conjugated Fluorene Moieties
期刊论文
Chinese Journal of Polymer Science, 2019, 卷号: Vol.37 No.4, 页码: 416-427
作者:
Yi-Wu Liu
;
Li-Shuang Tang
;
Lun-Jun Qu
;
Si-Wei Liu
;
Zhen-Guo Chi
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浏览/下载:112/0
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提交时间:2019/12/13
Functional polyimide
Fluorene derivative moieties
Fluorescence polymer
Low dielectric constant
Thermal stability
Structure effect on transition mechanism of UV-visible absorption spectrum in polyimides: A density functional theory study
期刊论文
POLYMER, 2018, 卷号: 148, 页码: 356-369
作者:
Ma, YP
;
Hu, CC
;
Guo, HX
;
Fan, L
;
Yang, SY
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浏览/下载:22/0
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提交时间:2019/04/08
Transition mechanism
DFT and TDDFT
Transparent polyimide
Restickable Oxide Neuromorphic Transistors with Spike-Timing-Dependent Plasticity and Pavlovian Associative Learning Activities
期刊论文
ADVANCED FUNCTIONAL MATERIALS, 2018, 卷号: 28, 期号: 44
作者:
Zhu, Li Qiang
;
Yu, Fei
;
Xiao, Hui
;
Gao, Wan Tian
;
Guo, Yan Bo
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浏览/下载:24/0
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提交时间:2018/12/04
Synaptic Plasticity
Chitosan Membranes
Skin Electronics
Synapses
Dog
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