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Modulating Charge Transport from Thermally Activated to "Band-Like" Through Interfacial Bottom-Up Binding Capability of Bilayer Polymer Dielectrics¥Y. Zheng, H. Lin, T. Jiang, D. Zhu, S. Qi, W. Li, L. Li, D. Ji and W. Hu¥2022¥1616301X¥The disordered chain arrangement of polymer dielectrics has complex both internal and external effects on system performance, which generally stimulates the weak acquisition and grain boundaries of vapor-deposited organic small molecule films (VDOSMFs) with thermally activated charge transport. As a result, achieving "band-like" transmission of VDOSMs on polymer dielectrics is attempting to prove to be a major challenge. Three types of bi-polymer dielectrics are developed to modulate charge transport from thermally activated mode to "band-like" transport at the interfacial level. The bottom consisting of a polyimide layer is critical to interfacial modulation, which shows the selectively binding capability with up-dielectric layers to realize the modulation of charge transport, as corroborated by interface characterization and density functional-based tight-binding calculation. The findings provide an effective strategy for modulating the charge transport through polymer dielectric engineering and also recommend a podium to further comprehend the electrical characteristics of small molecules in organic thin-film transistors. 2022 Wiley-VCH GmbH.¥internal-pdf://1153944661/Modulating Charge Transport from Thermally Act.pdf¥10.1002/adfm.202211742¥https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202211742?download=true¥ei 期刊论文
1616301X, 2022
作者:  Y. Zheng;  H. Lin;  T. Jiang;  D. Zhu;  S. Qi
收藏  |  浏览/下载:1/0  |  提交时间:2023/06/14
Modulating Charge Transport from Thermally Activated to "Band-Like" Through Interfacial Bottom-Up Binding Capability of Bilayer Polymer Dielectrics 期刊论文
1616301X, 2022
作者:  Y. Zheng;  H. Lin;  T. Jiang;  D. Zhu;  S. Qi
收藏  |  浏览/下载:1/0  |  提交时间:2023/07/17
A simple strategy to prepare functional PI microspheres by constructing coating on PAA microspheres followed thermal imidization reaction 期刊论文
COMPOSITES COMMUNICATIONS, 2021, 卷号: 24
作者:  Zhang, Qian;  Han, Yazhe;  Ding, Xin;  Zhang, Ping;  Wang, Yanyan
收藏  |  浏览/下载:43/0  |  提交时间:2021/05/06
Imidization-induced carbon nitride nanosheets orientation towards highly thermally conductive polyimide film with superior flexibility and electrical insulation 期刊论文
COMPOSITES PART B-ENGINEERING, 2020, 卷号: 199
作者:  Wang, Yanyan;  Zhang, Xian;  Ding, Xin;  Zhang, Ping;  Shu, Mengting
收藏  |  浏览/下载:65/0  |  提交时间:2020/11/30
Thermally rearranged polymer membranes containing highly rigid biphenyl ortho-hydroxyl diamine for hydrogen separation 期刊论文
JOURNAL OF MEMBRANE SCIENCE, 2020, 卷号: 604, 页码: 12
作者:  Hu, Xiaofan;  Lee, Won Hee;  Zhao, Jiayi;  Kim, Ju Sung;  Wang, Zhen
收藏  |  浏览/下载:17/0  |  提交时间:2020/09/22
Modeling Gas and Vapor Sorption and Swelling in Triptycene-Based Polybenzoxazole: Evidence for Entropy-Driven Sorption Behavior 期刊论文
MACROMOLECULES, 2019, 卷号: 52, 期号: 11, 页码: 4385-4395
作者:  Loianno, Valerio;  Zhang, Qinnan;  Luo, Shuangjiang;  Guo, Ruilan;  Galizia, Michele
收藏  |  浏览/下载:44/0  |  提交时间:2019/09/03
Polarization-induced alignment of azobenzene/fluorinated polyimide for three-dimensional shape-persistent and photo-responsive elastic helixes 期刊论文
Composites Science and Technology, 2019, 卷号: Vol.169, 页码: 158-166
作者:  Li, S.;  Feng, Y.;  Wang, W.;  Ji, T.;  Han, J.
收藏  |  浏览/下载:9/0  |  提交时间:2019/11/21
Synthesis and Properties of High Performance Functional Polyimides Containing Rigid Nonplanar Conjugated Fluorene Moieties 期刊论文
Chinese Journal of Polymer Science, 2019, 卷号: Vol.37 No.4, 页码: 416-427
作者:  Yi-Wu Liu;  Li-Shuang Tang;  Lun-Jun Qu;  Si-Wei Liu;  Zhen-Guo Chi
收藏  |  浏览/下载:112/0  |  提交时间:2019/12/13
Structure effect on transition mechanism of UV-visible absorption spectrum in polyimides: A density functional theory study 期刊论文
POLYMER, 2018, 卷号: 148, 页码: 356-369
作者:  Ma, YP;  Hu, CC;  Guo, HX;  Fan, L;  Yang, SY
收藏  |  浏览/下载:22/0  |  提交时间:2019/04/08
Restickable Oxide Neuromorphic Transistors with Spike-Timing-Dependent Plasticity and Pavlovian Associative Learning Activities 期刊论文
ADVANCED FUNCTIONAL MATERIALS, 2018, 卷号: 28, 期号: 44
作者:  Zhu, Li Qiang;  Yu, Fei;  Xiao, Hui;  Gao, Wan Tian;  Guo, Yan Bo
收藏  |  浏览/下载:24/0  |  提交时间:2018/12/04


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