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基于高分辨质谱的土壤溶解性有机质化学多样性研究 学位论文
北京: 中国科学院生态环境研究中心, 2018
作者:  李晓明
收藏  |  浏览/下载：24/0  |  提交时间：2020/07/15
土壤溶解性有机质， 化学多样性，微生物多样性， 傅立叶变换离子回旋 共振质谱  decreased WIth IncreasIng Iron ComplexIng Index. PAtterns In Molecular PrOfiles IndicAted Dom In Paddy Soils To Become More RecalcItrAnt At Higher Soil C/n rAtio And Higher Soil Ph. furTherMore, PlAnt-derived polyPh.nols And Pyrogenic Dom Were retaIned Favorably By Iron And The ChemodiversIty Of Dom In Paddy Soil Increased WIth IncreasIng Soil C/n rAtios. These Results Provide Novel InFormAtion regardIng Dom Characteristics At a Molecular Level And Will InForm Better Global MAnagement Of Soil Carbon In Paddy Soil EcosysteMs Global. 2) Through The applicAtion Of Ft-icr-Ms, The ChemodiversIty Of Dom In Soil Subjected To Long-term OrgAnic Carbon And InOrgAnic Fertilizer Amendments Was Established. In Parallel, Bcc Was Assessed. Through This Coupled Approach It Was Established.thAt sustaIned OrgAnic Carbon Amendment Resulted In: SignificAntly (p < 0.05) Increased Total Carbon And Total nItrogen Reservoirs In Soil, Dom PrOfiles Of greAter ChemodiversIty, And Emergence Of RecalcItrAnt Dom Moieties (H/c < 1.5). In Contrast, Carbon And nItrogen Reservoirs In Soil Subjected To sustaIned InOrgAnic Fertilizer applicAtion Were Unaltered, While Soil OrgAnic Carbon ChemodiversIty Was Observed To Shift To Less RecalcItrAnt Dom Moieties (H/c rAtio > 1.5 And O/c rAtios < 0.5). furTherMore, sustaIned OrgAnic Carbon Amendment Shaped Bcc To a eutroPh.c stAte While Long-term Chemical fertilizAtion Directed The Bcc Towards An oligotroPh.c stAte. Higher connectivIty And Network complexIty Were Observed In OrgAnic Carbon Amended Soils. Dom-Bcc Network Analysis, IndicAtIng thAt Soil Microbes Had More Interaction WIth Dom Molecules followIng sustaIned OrgAnic mAtter Input. These Results Highlight The Potential For OrgAnic Carbon Amendments To Not Only Build Soil Carbon sTocks And Increase Their Resilience, But To Also Improve The Functional stAte Of Soil Microbial communIties. Key Words: Dom, ChemodiversIty, Microbial diversIty, Ft-icr Ms  
Facet-Mediated Adsorption and Molecular Fractionation of Humic Substances on Hematite Surfaces 期刊论文
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2018, 卷号: 52, 期号: 20, 页码: 11660-11669
作者:  Lv, Jitao;  Miao, Yuexia;  Huang, Zaoquan;  Han, Ruixia;  Zhang, Shuzhen
收藏  |  浏览/下载：28/0  |  提交时间：2019/06/20
Formation of organobromine and organoiodine compounds by engineered TiO2 nanoparticle-induced photohalogenation of dissolved organic matter in environmental waters 期刊论文
SCIENCE OF THE TOTAL ENVIRONMENT, 2018, 卷号: 631-632, 页码: 158-168
作者:  Hao, Zhineng;  Yin, Yongguang;  Wang, Juan;  Cao, Dong;  Liu, Jingfu
收藏  |  浏览/下载：37/0  |  提交时间：2019/06/20
Sources, compositions, and optical properties of humic-like substances in Beijing during the 2014 APEC summit: Results from dual carbon isotope and Fourier-transform ion cyclotron resonance mass spectrometry analyses 期刊论文
ENVIRONMENTAL POLLUTION, 2018, 卷号: 239, 页码: 322-331
作者:  Mo, Yangzhi;  Li, Jun;  Jiang, Bin;  Su, Tao;  Geng, Xiaofei
收藏  |  浏览/下载：19/0  |  提交时间：2020/07/08
Characterization of brominated disinfection byproducts formed during chloramination of fulvic acid in the presence of bromide 期刊论文
SCIENCE OF THE TOTAL ENVIRONMENT, 2018, 卷号: 627, 期号: 0, 页码: 118-124
作者:  Zhang, Haifeng;  Yang, Min
收藏  |  浏览/下载：18/0  |  提交时间：2019/06/21
Comprehensive Characterization of Swine Cardiac Troponin T Proteoforms by Top-Down Mass Spectrometry 期刊论文
JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY, 2018, 卷号: 29, 期号: 6, 页码: 1284-1294
作者:  Lin, Ziqing;  Guo, Fang;  Gregorich, Zachery R.;  Sun, Ruixiang;  Zhang, Han
收藏  |  浏览/下载：29/0  |  提交时间：2019/12/10
Characterization of Brominated Disinfection Byproducts Formed During the Chlorination of Aquaculture Seawater 期刊论文
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2018, 卷号: 52, 期号: 10, 页码: 5662-5670
作者:  Wang, Juan;  Hao, Zhineng;  Shi, Fengqiong;  Yin, Yongguang;  Cao, Dong
收藏  |  浏览/下载：38/0  |  提交时间：2019/06/20
Abiotic formation of organoiodine compounds by manganese dioxide induced iodination of dissolved organic matter 期刊论文
ENVIRONMENTAL POLLUTION, 2018, 卷号: 236, 页码: 672-679
作者:  Hao, Zhineng;  Wang, Juan;  Yin, Yongguang;  Cao, Dong;  Liu, Jingfu
收藏  |  浏览/下载：26/0  |  提交时间：2019/06/20
Relationship between Molecular Components and Reducing Capacities of Humic Substances 期刊论文
ACS EARTH AND SPACE CHEMISTRY, 2018, 卷号: 2, 期号: 4, 页码: 330-339
作者:  Lv, Jitao;  Cao, Dong;  Han, Ruixia;  Huang, Zaoquan;  Zhang, Shuzhen
收藏  |  浏览/下载：40/0  |  提交时间：2019/06/20
Molecular Chemodiversity of Dissolved Organic Matter in Paddy Soils 期刊论文
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2018, 卷号: 52, 期号: 3, 页码: 963-971
作者:  Sun, Guo-Xin;  Li, Xiao-Ming;  Chen, Song-Can;  Fang, Zhi;  Yuan, Hai-Yan
收藏  |  浏览/下载：38/0  |  提交时间：2019/06/17

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