Thermally treated 3-D nanostructured graphene-supported Pd catalyst for significantly improved electrocatalytic performance towards ethanol electrooxidation

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	Thermally treated 3-D nanostructured graphene-supported Pd catalyst for significantly improved electrocatalytic performance towards ethanol electrooxidation
	Wu, Li Juan 1,2; Wang, Yi 1; Wang, Yan Ping 2; Du, Xuan 1; Wang, Fang 1; Gao, Yi Ying 1; Qi, Tao 1; Li, Chang Ming 3,4,5
刊名	RSC ADVANCES
	2013
卷号	3 期号:15 页码:5196-5203
英文摘要	Catalyst supports are known to play a critical role in high catalytic performance. A novel nanostructured graphene was obtained by facile thermal treatment of the three-dimensional (3-D) graphene material. X-ray diffraction (XRD), scanning electron microscopy (SEM) and nitrogen adsorption results reveal that the new material is composed of smaller and looser graphene nanosheets, and possesses an ultrahigh specific surface area, large pore volume and rich 3-D interconnected macropores and mesopores. The material was further used to support a Pd catalyst towards ethanol electrooxidation in alkaline media, demonstrating much better electrocatalytic activity in respect of the Pd utility ratio, onset potential and peak current density than that of pristine 3-D graphene material and carbon black, the most popular catalyst support, and thus rendering a promising catalyst support material for fuel cells.
WOS标题词	Science & Technology ; Physical Sciences
类目[WOS]	Chemistry, Multidisciplinary
研究领域[WOS]	Chemistry
关键词[WOS]	METHANOL FUEL-CELLS ; OXYGEN REDUCTION ; CARBON NANOTUBES ; ACTIVATED CARBON ; ALKALINE MEDIA ; OXIDATION ; MEMBRANE ; PLATINUM ; SURFACE
收录类别	SCI
语种	英语
WOS记录号	WOS:000316226500046
公开日期	2015-05-27
内容类型	期刊论文
源URL	[http://ir.ipe.ac.cn/handle/122111/13665]
专题	过程工程研究所_研究所（批量导入）
作者单位	1.Chinese Acad Sci, Natl Engn Lab Hydromet Cleaner Prod Technol, Inst Proc Engn, Beijing 100190, Peoples R China 2.Inner Mongolia Polytech Univ, Sch Chem Engn, Hohhot 010051, Peoples R China 3.Nanyang Technol Univ, Sch Chem & Biomed Engn, Singapore 637457, Singapore 4.Southwest Univ, Inst Clean Energy & Adv Mat, Chongqing 400715, Peoples R China 5.Chongqing Key Lab Adv Mat & Technol Clean Energie, Chongqing 400715, Peoples R China
推荐引用方式 GB/T 7714	Wu, Li Juan,Wang, Yi,Wang, Yan Ping,et al. Thermally treated 3-D nanostructured graphene-supported Pd catalyst for significantly improved electrocatalytic performance towards ethanol electrooxidation[J]. RSC ADVANCES,2013,3(15):5196-5203.
APA	Wu, Li Juan.,Wang, Yi.,Wang, Yan Ping.,Du, Xuan.,Wang, Fang.,...&Li, Chang Ming.(2013).Thermally treated 3-D nanostructured graphene-supported Pd catalyst for significantly improved electrocatalytic performance towards ethanol electrooxidation.RSC ADVANCES,3(15),5196-5203.
MLA	Wu, Li Juan,et al."Thermally treated 3-D nanostructured graphene-supported Pd catalyst for significantly improved electrocatalytic performance towards ethanol electrooxidation".RSC ADVANCES 3.15(2013):5196-5203.