Connection between Mechanical Relaxation and Equilibration Kinetics in a High-Entropy Metallic Glass

doi:10.1103/PhysRevLett.132.056101

CORC > 力学研究所 > 中国科学院力学研究所 > 非线性力学国家重点实验室

	Connection between Mechanical Relaxation and Equilibration Kinetics in a High-Entropy Metallic Glass
	Duan, Y. J.10,11; Nabahat, M.10; Tong, Yu 8,9; Ortiz-Membrado, L.7; Jimenez-Pique, E.7; Zhao, Kun 5,6; Wang, Yun-Jiang 5,6; Yang, Y.3,4; Wada, T.2; Kato, H.2
刊名	PHYSICAL REVIEW LETTERS
	2024-01-29
卷号	132 期号:5 页码:7
ISSN号	0031-9007
DOI	10.1103/PhysRevLett.132.056101
通讯作者	Qiao, J. C.(qjczy@nwpu.edu.cn) ; Pineda, E.(eloi.pineda@upc.edu)
英文摘要	The slow transition from an out-of-equilibrium glass towards a supercooled liquid is a complex relaxation phenomenon. In this Letter, we study the correlation between mechanical relaxation and equilibration kinetics in a Pd20Pt20Cu20Ni20P20 high-entropy metallic glass. The evolution of stress relaxation with aging time was obtained with an unprecedented detail, allowing us to pinpoint new interesting features. The long structural relaxation towards equilibrium contains a wide distribution of activation energies, instead of being just associated to the beta relaxation as commonly accepted. The stress relaxation time can be correlated with the equilibration rate and we observe a decrease of microstructural heterogeneity which contrasts with an increase of dynamic heterogeneity. These results significantly enhance our insight of the interplay between relaxation dynamics and thermodynamics in metallic glasses.
资助项目	NSFC[51971178] ; NSFC[52271153] ; NSFC[12072344] ; Natural Science Basic Research Plan for Distinguished Young Scholars in Shaanxi Province[2021JC-12] ; Fundamental Research Funds for the Central Universities[D5000220034] ; FY2023 GIMRT[202212-RDKGE-0504] ; Youth Innovation Promotion Association of the Chinese Academy of Sciences ; Research Grant Council (RGC) ; Hong Kong government through the General Research Fund (GRF)[CityU11206362] ; Hong Kong government through the General Research Fund (GRF)[CityU11201721] ; MCIN/AEI[PID2020-112975GB-I00] ; MCIN/AEI[PID2021-126614OB-I00] ; Generalitat de Catalunya ; AGAUR[2021SGR00343] ; Innovation Foundation for Doctor Dissertation of Northwestern Polytechnical University[CX202031] ; China Scholarship Council (CSC)[202006290092]
WOS关键词	BETA-RELAXATION ; SPATIAL HETEROGENEITY ; SECONDARY RELAXATION ; ELASTIC-MODULUS ; INDENTATION ; BEHAVIOR ; DYNAMICS ; REJUVENATION ; TRANSITION ; HARDNESS
WOS研究方向	Physics
语种	英语
WOS记录号	WOS:001181999900002
资助机构	NSFC ; Natural Science Basic Research Plan for Distinguished Young Scholars in Shaanxi Province ; Fundamental Research Funds for the Central Universities ; FY2023 GIMRT ; Youth Innovation Promotion Association of the Chinese Academy of Sciences ; Research Grant Council (RGC) ; Hong Kong government through the General Research Fund (GRF) ; MCIN/AEI ; Generalitat de Catalunya ; AGAUR ; Innovation Foundation for Doctor Dissertation of Northwestern Polytechnical University ; China Scholarship Council (CSC)
内容类型	期刊论文
源URL	[http://dspace.imech.ac.cn/handle/311007/94881]
专题	力学研究所_非线性力学国家重点实验室
通讯作者	Qiao, J. C.; Pineda, E.
作者单位	1.Univ Lyon, MATEIS, CNRS, UMR 5510,INSA Lyon, Batiment Blaise Pascal, F-69621 Lyon, France 2.Tohoku Univ, Inst Mat Res, Sendai 9808577, Japan 3.City Univ Hong Kong, Coll Engn, Dept Mat Sci & Engn, Tat Chee Ave,Kowloon Tong, Hong Kong, Peoples R China 4.City Univ Hong Kong, Coll Engn, Dept Mech Engn, Tat Chee Ave,Kowloon Tong, Hong Kong, Peoples R China 5.Univ Chinese Acad Sci, Sch Engn Sci, Beijing 100049, Peoples R China 6.Chinese Acad Sci, Inst Mech, State Key Lab Nonlinear Mech, Beijing 100190, Peoples R China 7.Univ Politecn Cataluna, Dept Mat Sci, Barcelona 08019, Spain 8.Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Zhejiang Prov Key Lab Magnet Mat & Applicat Techno, Ningbo 315201, Peoples R China 9.Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, CAS Key Lab Magnet Mat & Devices, Ningbo 315201, Peoples R China 10.Univ Politecn Cataluna, Inst Energy Technol, Dept Phys, Barcelona 08019, Spain
推荐引用方式 GB/T 7714	Duan, Y. J.,Nabahat, M.,Tong, Yu,et al. Connection between Mechanical Relaxation and Equilibration Kinetics in a High-Entropy Metallic Glass[J]. PHYSICAL REVIEW LETTERS,2024,132(5):7.
APA	Duan, Y. J..,Nabahat, M..,Tong, Yu.,Ortiz-Membrado, L..,Jimenez-Pique, E..,...&Pineda, E..(2024).Connection between Mechanical Relaxation and Equilibration Kinetics in a High-Entropy Metallic Glass.PHYSICAL REVIEW LETTERS,132(5),7.
MLA	Duan, Y. J.,et al."Connection between Mechanical Relaxation and Equilibration Kinetics in a High-Entropy Metallic Glass".PHYSICAL REVIEW LETTERS 132.5(2024):7.