Advances and Prospects of Supercritical CO<sub>2</sub> for Shale Gas Extraction and Geological Sequestration in Gas Shale Reservoirs

doi:10.1021/acs.energyfuels.3c03843

CORC > 力学研究所 > 中国科学院力学研究所 > 流固耦合系统力学重点实验室(2012-)

	Advances and Prospects of Supercritical CO₂ for Shale Gas Extraction and Geological Sequestration in Gas Shale Reservoirs
	Shen WJ(沈伟军); Ma, Tianran; Zuo, Luo; Yang X(杨旭); Cai, Jianchao
刊名	ENERGY & FUELS
	2024-01-09
卷号	38 期号:2 页码:789-805
ISSN号	0887-0624
DOI	10.1021/acs.energyfuels.3c03843
通讯作者	Shen, Weijun(wjshen763@imech.ac.cn) ; Cai, Jianchao(caijc@cup.edu.cn)
英文摘要	The advancements in hydraulic fracturing and horizontal drilling techniques have substantially facilitated the large-scale extraction of natural gas from shale gas reservoirs. However, the use of fracking water poses several potential drawbacks including the contamination of groundwater, surface water, and soil, as well as risks to air quality. Due to the unique physical properties of supercritical CO2, shale gas exploitation using this method has been considered a promising technology that can not only improve gas recovery but can also enable CO2 geological storage. This paper clarifies the gas adsorption mechanism in shale formations, including the factors influencing the adsorption of CH4, the differences between CH4 and CO2 adsorption, and various adsorption models. We show that shale inherently exhibits a preference for CO2 adsorption over CH4. Then, the supercritical CO2 fracturing mechanism, including the shale fracking pressure and the factors influencing CO2 fracturing, is analyzed. The mechanisms of CO2 extraction in shale gas and the key factors influencing CO2 geological storage are discussed. The main challenges and future prospects regarding the use of supercritical CO2 for shale gas recovery and geological sequestration in gas shale reservoirs are finally summarized. A more detailed understanding is required to evaluate the efficiency of shale gas recovery and CO2 geological sequestration in shale formations using supercritical CO2. This work provides a basis and serves as a reference for future research investigating the mechanisms of shale gas exploitation using supercritical CO2, as well as the limitations and advantages of CO2 geological sequestration in unconventional shale gas reservoirs.
分类号	二类/Q1
资助项目	National Natural Science Foundation of China[12172362] ; National Natural Science Foundation of China[2021DQ02-0204] ; China National Petroleum Corporation (CNPC) Innovation Fund[2023024] ; Youth Innovation Promotion Association of Chinese Academy of Sciences
WOS关键词	CO2/CH4 COMPETITIVE ADSORPTION ; CARBON-DIOXIDE ; METHANE ADSORPTION ; PORE STRUCTURE ; VANDERWAALS FORCES ; REACTIVE TRANSPORT ; STORAGE CAPACITY ; RESIDUAL-GAS ; FLOW ; BASIN
WOS研究方向	Energy & Fuels ; Engineering
语种	英语
WOS记录号	WOS:001145487800001
资助机构	National Natural Science Foundation of China ; National Natural Science Foundation of China ; China National Petroleum Corporation (CNPC) Innovation Fund ; Youth Innovation Promotion Association of Chinese Academy of Sciences
其他责任者	Shen, Weijun ; Cai, Jianchao
内容类型	期刊论文
源URL	[http://dspace.imech.ac.cn/handle/311007/94148]
专题	力学研究所_流固耦合系统力学重点实验室(2012-)
推荐引用方式 GB/T 7714	Shen WJ,Ma, Tianran,Zuo, Luo,et al. Advances and Prospects of Supercritical CO₂ for Shale Gas Extraction and Geological Sequestration in Gas Shale Reservoirs[J]. ENERGY & FUELS,2024,38(2):789-805.
APA	沈伟军,Ma, Tianran,Zuo, Luo,杨旭,&Cai, Jianchao.(2024).Advances and Prospects of Supercritical CO₂ for Shale Gas Extraction and Geological Sequestration in Gas Shale Reservoirs.ENERGY & FUELS,38(2),789-805.
MLA	沈伟军,et al."Advances and Prospects of Supercritical CO₂ for Shale Gas Extraction and Geological Sequestration in Gas Shale Reservoirs".ENERGY & FUELS 38.2(2024):789-805.