Upward trend and formation of surface ozone in the Guanzhong Basin, Northwest China
Xue, Yonggang1,2,3; Wang, Liqin1,2,3; Liu, Suixin1,2,3; Huang, Yu1,2,3; Chen, Long1,2,3; Cui, Long1,2,3; Cao, Junji1,2,3
刊名JOURNAL OF HAZARDOUS MATERIALS
2022-04-05
卷号427页码:9
关键词Ozone VOCs Regional transport Traffic exhaust
ISSN号0304-3894
DOI10.1016/j.jhazmat.2021.128175
通讯作者Huang, Yu(huangyu@ieecas.cn)
英文摘要Increase trend of surface ozone (O-3) was observed in the Guanzhong Basin (GZB) from 2014 to 2020 with growth rates of 3.9-6.4 mu g M-3 yr(-1) for the maximum daily average 8 h (MDA8) O-3 concentrations. To further understand the formation of O-3 , investigation of volatile organic compounds (VOCs) was carried out in the summer of 2018. High levels of VOCs were observed in both residential area and industrialized cities. Elevated concentrations of none-methane Hydrocarbon (NMHCs) were observed in rush hours, which indicated dominated roles of traffic activities on the loading of ambient VOCs. In the nighttime, both of NMHCs and oxygenated VOCs (OVOCs) were raised, and the peaks of VOCs kept pace with accumulation of O-3 . Wind field indicated that northward and westward air mass, which passed through the remote forest and industrial area in east of the GZB, was responsible to elevated ambient VOCs in the GZB. Traffic emission, fuel evaporation, and solvent using were key contributors to ambient NMHCs, while solvent using and secondary formation dominated the loading of OVOCs. The present study indicated that both local management and regional collaborative control on active VOCs species from typical sources is urgently needed in GZB.
资助项目National Key Research and Devel-opment Program of China[2017YFC0212200] ; National Key Research and Devel-opment Program of China[2016YFA0203000] ; National Natural Science Foundation of China[41701565] ; National Natural Science Foundation of China[41877308] ; CAS Light of West China Program[XAB2019B06]
WOS关键词VOLATILE ORGANIC-COMPOUNDS ; COMPOUNDS VOCS ; DIURNAL-VARIATIONS ; CARBONYL-COMPOUNDS ; REACTIVITY SCALES ; SECONDARY SOURCES ; AIR-POLLUTION ; SUMMER OZONE ; URBAN SITE ; IMPACT
WOS研究方向Engineering ; Environmental Sciences & Ecology
语种英语
出版者ELSEVIER
WOS记录号WOS:000752556900004
资助机构National Key Research and Devel-opment Program of China ; National Natural Science Foundation of China ; CAS Light of West China Program
内容类型期刊论文
源URL[http://ir.ieecas.cn/handle/361006/17466]  
专题地球环境研究所_粉尘与环境研究室
通讯作者Huang, Yu
作者单位1.Guanzhong Plain Ecol Environm Change & Comprehens, Xian 710061, Peoples R China
2.CAS Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Peoples R China
3.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol SKLLQG, Xian 710061, Peoples R China
推荐引用方式
GB/T 7714
Xue, Yonggang,Wang, Liqin,Liu, Suixin,et al. Upward trend and formation of surface ozone in the Guanzhong Basin, Northwest China[J]. JOURNAL OF HAZARDOUS MATERIALS,2022,427:9.
APA Xue, Yonggang.,Wang, Liqin.,Liu, Suixin.,Huang, Yu.,Chen, Long.,...&Cao, Junji.(2022).Upward trend and formation of surface ozone in the Guanzhong Basin, Northwest China.JOURNAL OF HAZARDOUS MATERIALS,427,9.
MLA Xue, Yonggang,et al."Upward trend and formation of surface ozone in the Guanzhong Basin, Northwest China".JOURNAL OF HAZARDOUS MATERIALS 427(2022):9.
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