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La(OH)(3) loaded magnetic nanocomposites derived from sugarcane bagasse cellulose for phosphate adsorption: Characterization, performance and mechanism
Wang, Yajun1; Li, Jinshou1; Yuan, Yan1; Si, Yunmei1; Xu, Jiaxiang2; Li, Mingxin2; Peng, Xiaoming2
刊名COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
2021-10-05
卷号626
关键词Magnetic nanomaterials Phosphate Model Response surface design Adsorption mechanism
ISSN号0927-7757
DOI10.1016/j.colsurfa.2021.127060
英文摘要The magnetic nanomaterials Mg-Al-La LDH/Fe3O4/C were prepared using Fe3O4/C as a precursor by hydrothermal and co-precipitation method, and served as adsorbents for the efficient uptake of phosphorus from aqueous solutions. The effects of adsorbent dosage, pH and co-existing ions on the adsorption of phosphate were studied. The adsorption performance of the material was described by the adsorption kinetic model, isothermal model and thermodynamic model. When the pH value of the solution is in 4-7, it shows a high phosphate removal rate (>98.7%). The maximum phosphate removal rate (99.43%) was obtained at pH=6. The phosphate adsorption process by Mg-Al-La LDH/Fe3O4/C was best described by the Langmuir isotherm model and pseudosecond-order reaction kinetics. The maximum adsorption capacity for phosphate was evaluated as 106.21 mg/g. The optimization of phosphate adsorption was carried out by response surface design. The adsorption mechanism of Mg-Al-La LDH/Fe3O4/C for phosphate could be explained by ion exchange, electrostatic attraction and ligand exchange. Experiments have proved that Mg-Al-La LDH/Fe3O4/C nanocomposite can be used as a potential material for adsorbing phosphate in polluted water.
WOS研究方向Chemistry
语种英语
出版者ELSEVIER
WOS记录号WOS:000685958800002
内容类型期刊论文
源URL[http://ir.lut.edu.cn/handle/2XXMBERH/148810]  
专题土木工程学院
作者单位1.Lanzhou Univ Technol, Sch Civil Engn, Lanzhou 730000, Gansu, Peoples R China;
2.East China Jiaotong Univ, Sch Civil Engn & Architecture, Nanchang 330013, Jiangxi, Peoples R China
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Wang, Yajun,Li, Jinshou,Yuan, Yan,et al. La(OH)(3) loaded magnetic nanocomposites derived from sugarcane bagasse cellulose for phosphate adsorption: Characterization, performance and mechanism[J]. COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS,2021,626.
APA Wang, Yajun.,Li, Jinshou.,Yuan, Yan.,Si, Yunmei.,Xu, Jiaxiang.,...&Peng, Xiaoming.(2021).La(OH)(3) loaded magnetic nanocomposites derived from sugarcane bagasse cellulose for phosphate adsorption: Characterization, performance and mechanism.COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS,626.
MLA Wang, Yajun,et al."La(OH)(3) loaded magnetic nanocomposites derived from sugarcane bagasse cellulose for phosphate adsorption: Characterization, performance and mechanism".COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS 626(2021).
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