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Construction of an efficient Z-scheme CuS/BiOBr heterojunction photocatalysts for dye degradation and Cr(VI) reduction
Di, Lijing1; Gao, Yushu1; Xian, Tao1; Sun, Xiaofeng1; Li, Hongqin1; Yang, Hua2
刊名JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
2022-07-01
卷号33期号:20页码:16521-16537
关键词Bismuth compoundsBromine compoundsChromium compoundsHeterojunctionsNanoparticlesPhotocatalytic activityRhodium compounds % reductionsAcid orange 7AnchoringsDye degradationNanoplatesPhoto-catalytic removalPhotocatalytic degradationRemoval activityRhodamine-BSimulated sunlight
ISSN号0957-4522
DOI10.1007/s10854-022-08545-7
英文摘要In this work, an efficient Z-scheme CuS/BiOBr heterojunction photocatalysts were developed through anchoring the CuS nanoparticles on the surface of BiOBr nanoplates. Acid orange 7 (AO7), Rhodamine B (RhB), and Cr(VI) were selected as target reactant for the investigation of photocatalytic degradation and reduction ability for the sample irradiated by simulated sunlight. The experimental results imply that the CuS/BiOBr composite exhibits much higher photocatalytic removal activity than that of bare BiOBr. Further more, the photocatalytic activity of composite is highly related to the content of CuS, and the optimal photocatalytic efficiency is achieved by 12%CuS/BiOBr sample. On the other hand, the synergistic photocatalytic removal activity of CuS/BiOBr composite for the purification of mixture (AO7/Cr(VI)) was also evaluated under simulated sunlight irradiation. The separation rate of photogenerated charges in BiOBr can be effectively promoted after the decoration of CuS nanoparticles. The main active species play role in the photocatalytic degradation process of CuS/BiOBr composite was detected by trapping experiment. According to these results, the photocatalytic mechanism of Z-scheme CuS/BiOBr composite was proposed.
WOS研究方向Engineering ; Materials Science ; Physics
语种英语
出版者SPRINGER
WOS记录号WOS:000813781700008
内容类型期刊论文
源URL[http://ir.lut.edu.cn/handle/2XXMBERH/158897]  
专题理学院
作者单位1.Qinghai Normal Univ, Coll Phys & Elect Informat Engn, Xining 810008, Peoples R China;
2.Lanzhou Univ Technol, State Key Lab Adv Proc & Recycling Nonferrous Met, Lanzhou 730050, Peoples R China
推荐引用方式
GB/T 7714
Di, Lijing,Gao, Yushu,Xian, Tao,et al. Construction of an efficient Z-scheme CuS/BiOBr heterojunction photocatalysts for dye degradation and Cr(VI) reduction[J]. JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS,2022,33(20):16521-16537.
APA Di, Lijing,Gao, Yushu,Xian, Tao,Sun, Xiaofeng,Li, Hongqin,&Yang, Hua.(2022).Construction of an efficient Z-scheme CuS/BiOBr heterojunction photocatalysts for dye degradation and Cr(VI) reduction.JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS,33(20),16521-16537.
MLA Di, Lijing,et al."Construction of an efficient Z-scheme CuS/BiOBr heterojunction photocatalysts for dye degradation and Cr(VI) reduction".JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS 33.20(2022):16521-16537.
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