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The mosaic structure design to improve the anchoring strength of SiOx@C@Graphite anode
Dong, H.1,2,3; Wang, J.2; Ding, H.2; Wang, P.2; Song, R.2; Zhang, N.2,3; Li, F.1,4; Li, S.1,2,3
刊名MATERIALS TODAY CHEMISTRY
2021-12
卷号22
关键词SiOx@C@Graphite anodes Bonding strength High performance
ISSN号2468-5194
DOI10.1016/j.mtchem.2021.100599
英文摘要Silicon oxide (SiOx)-based anodes have aroused great interest as the most promising alternative anode in the practical application of high-performance lithium-ion batteries. However, the electrochemical performance is inhibited because of the large volume change, and the electrode structure deteriorates during the cycling process, which hinders their practical application. In this article, a novel fabrication method for the synthesis of high-performance SiOx@C@Graphite composites is presented. SiOx particles are anchored on the graphite surface by chemical vapor deposition and compression molding. This structure makes up the shortcomings of poor electrical conductivity and poor bonding strength between SiOx and graphite particles. It is beneficial to form a stable solid electrolyte interface and helps to maintain the structural integrity of electrode materials. As a result, the synthetic SiOx@C@Graphite anode shows a high reversible capacity (2698.8 mA h), excellent cycle stability (about 76.9% capacity retention for 500 cycles) and a superior rate ability. Our research hopes to provide a new idea for improving the bonding strength of the surface coating. (C) 2021 Elsevier Ltd. All rights reserved.
WOS研究方向Chemistry ; Materials Science
语种英语
出版者ELSEVIER SCI LTD
WOS记录号WOS:000708675900003
内容类型期刊论文
源URL[http://ir.lut.edu.cn/handle/2XXMBERH/150110]  
专题材料科学与工程学院
作者单位1.Lanzhou Univ Technol, Sch Petrochem Technol, Lanzhou 730050, Peoples R China;
2.Key Lab Low Carbon Energy & Chem Engn Gansu Prov, Lanzhou 730050, Peoples R China;
3.Gansu Engn Lab Cathode Mat Lithium Ion Battery, Lanzhou 730050, Peoples R China;
4.Linyi Univ, Sch Mat Sci & Engn, Linyi 276005, Peoples R China
推荐引用方式
GB/T 7714
Dong, H.,Wang, J.,Ding, H.,et al. The mosaic structure design to improve the anchoring strength of SiOx@C@Graphite anode[J]. MATERIALS TODAY CHEMISTRY,2021,22.
APA Dong, H..,Wang, J..,Ding, H..,Wang, P..,Song, R..,...&Li, S..(2021).The mosaic structure design to improve the anchoring strength of SiOx@C@Graphite anode.MATERIALS TODAY CHEMISTRY,22.
MLA Dong, H.,et al."The mosaic structure design to improve the anchoring strength of SiOx@C@Graphite anode".MATERIALS TODAY CHEMISTRY 22(2021).
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