One-step method to achieve multiple decorations on lamellar MoS2 to synergistically enhance the electrocatalytic HER performance

doi:10.1016/j.jallcom.2020.155217

CORC > 兰州理工大学 > 兰州理工大学

	One-step method to achieve multiple decorations on lamellar MoS2 to synergistically enhance the electrocatalytic HER performance
	Lin, Zhiping 2; Wang, Zongpeng 2; Shen, Shijie 1,2; Chen, Yuchao 2; Du, Zexin 2; Tao, Weiying 2; Xu, Aijiao 2; Ye, Xiufang 3; Zhong, Wenwu 2; Feng, Shangshen 4
刊名	Journal of Alloys and Compounds
	2020-09-05
卷号	834
关键词	Catalyst activity Electrocatalysis Hydrogen evolution reaction Molybdenum compounds Pulsed lasers Electrocatalytic Electrocatalytic performance Laser treated Number of active sites One-step methods Overpotential Tafel slopes Ultrafast pulsed lasers
ISSN号	09258388
DOI	10.1016/j.jallcom.2020.155217
英文摘要	Lamellar MoS2 has attracted widespread attention as a potential electrocatalytic HER (Hydrogen evolution reaction) catalyst. However, it is difficult to further improve its catalytic activity due to two major drawbacks: the limited number of active sites and its poor conductivity. Here, we adopt a one-step method utilizing an ultrafast pulsed laser treatment to produce multiple decorations on lamellar MoS2, where nanocrystallization and amorphization of lamellar MoS2 are achieved simultaneously, along with an additional characteristic of atomic steps. Due to this special microstructure, laser-treated MoS2 exhibits excellent electrocatalytic performance with a low overpotential and a small Tafel slope (217 mV @ 10 mA cm−2 and 74.5 mV dec−1, respectively), which is superior to that of untreated lamellar MoS2 (461 mV @ 10 mA cm−2 and 142.6 mV dec−1, respectively). The MoS2 prepared in this way has a high catalytic activity and a high stability, which indicates potential for electrocatalysis applications. © 2020 Elsevier B.V.
WOS研究方向	Chemistry ; Materials Science ; Metallurgy & Metallurgical Engineering
语种	英语
出版者	Elsevier Ltd
WOS记录号	WOS:000534498700004
内容类型	期刊论文
源URL	[http://ir.lut.edu.cn/handle/2XXMBERH/115522]
专题	兰州理工大学材料科学与工程学院
作者单位	1.School of Materials Science and Engineering, Lanzhou University of Technology, Lanzhou; 730050, China; 2.School of Pharmaceutical and Materials Engineering, School of Advanced Study, Taizhou University, Taizhou; Zhejiang; 318000, China; 3.School of Materials Science and Energy Engineering, Foshan University, Foshan; 528225, China; 4.School of Science, Zhejiang A&F University, Hangzhou; Zhejiang; 311300, China
推荐引用方式 GB/T 7714	Lin, Zhiping,Wang, Zongpeng,Shen, Shijie,et al. One-step method to achieve multiple decorations on lamellar MoS2 to synergistically enhance the electrocatalytic HER performance[J]. Journal of Alloys and Compounds,2020,834.
APA	Lin, Zhiping.,Wang, Zongpeng.,Shen, Shijie.,Chen, Yuchao.,Du, Zexin.,...&Feng, Shangshen.(2020).One-step method to achieve multiple decorations on lamellar MoS2 to synergistically enhance the electrocatalytic HER performance.Journal of Alloys and Compounds,834.
MLA	Lin, Zhiping,et al."One-step method to achieve multiple decorations on lamellar MoS2 to synergistically enhance the electrocatalytic HER performance".Journal of Alloys and Compounds 834(2020).