Design and Synthesis of a Catalytically Active Cu-SSZ-13 Zeolite from a Copper-Amine Complex Template | |
Ren LM ; Zhang YB ; Zeng SJ ; Zhu LF ; Sun Q ; Zhang HY ; Yang CG ; Meng XJ ; Yang XG ; Xiao FS | |
刊名 | chinese journal of catalysis |
2012 | |
卷号 | 33期号:1页码:92-105 |
关键词 | STRUCTURE-DIRECTING AGENT METHANOL-TO-OLEFIN MOLECULAR-SIEVES METALLOALUMINOPHOSPHATES STA-6 IONOTHERMAL SYNTHESIS REDUCTION CATALYSTS ALUMINOPHOSPHATE FRAMEWORK NH3 |
ISSN号 | 0253-9837 |
通讯作者 | xiao fs |
中文摘要 | the modern synthesis of zeolites typically uses organic structure-directing agents. therefore, the developing of new templates is part of zeolite research. the design and synthesis of cu-ssz-13 using a novel template of a low-cost copper amine complex (cu2+ coordinated with tetraethylenepentamine) were reported, where the copper amine complex is both a template for synthesizing the ssz-13 structure and a source of copper species in the zeolite. the calculated size of the complex (0.728 nm x 0.922 nm) matches well with the cha cages (0.73 nm x 1.2 nm), which are the building units of the ssz-13 zeolite. various techniques were used to investigate the chemical and physical properties of the synthesized zeolite. the results showed that the sample has the ssz-13 zeolite structure, high crystallinity, adjustable si/al ratios, and controllable copper loading. catalytic tests using the selective catalytic reduction of nox with nh3 showed that the cu-ssz-13 was a superior catalyst, and it can be important for the abatement of environmentally harmful nox. |
收录类别 | SCI收录期刊论文 |
语种 | 英语 |
公开日期 | 2013-10-31 |
内容类型 | 期刊论文 |
源URL | [http://ir.ciac.jl.cn/handle/322003/48910] |
专题 | 长春应用化学研究所_长春应用化学研究所知识产出_期刊论文 |
推荐引用方式 GB/T 7714 | Ren LM,Zhang YB,Zeng SJ,et al. Design and Synthesis of a Catalytically Active Cu-SSZ-13 Zeolite from a Copper-Amine Complex Template[J]. chinese journal of catalysis,2012,33(1):92-105. |
APA | Ren LM.,Zhang YB.,Zeng SJ.,Zhu LF.,Sun Q.,...&Xiao FS.(2012).Design and Synthesis of a Catalytically Active Cu-SSZ-13 Zeolite from a Copper-Amine Complex Template.chinese journal of catalysis,33(1),92-105. |
MLA | Ren LM,et al."Design and Synthesis of a Catalytically Active Cu-SSZ-13 Zeolite from a Copper-Amine Complex Template".chinese journal of catalysis 33.1(2012):92-105. |
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