Iodine-assisted antisolvent engineering for stable perovskite solar cells with efficiency >21.3 % | |
F. Y. Wang,M. F. Yang,S. Yang,X. Qu,L. L. Yang,L. Fan,J. H. Yang and F. Rosei | |
刊名 | Nano Energy |
2020 | |
卷号 | 67页码:8 |
ISSN号 | 2211-2855 |
DOI | 10.1016/j.nanoen.2019.104224 |
英文摘要 | The quality of the photoactive film is a significant factor in determining the power conversion efficiency (PCE) and the stability of pemvskite solar cells (PSCs). We report a simple upgraded antisolvent washing treatment using iodine modulation, which significantly improves the MAPbI(3) films with high crystallinity and chemical uniformity. A detailed model for improving the mechanism is proposed to describe how the upgraded antisolvent enhances both the perovskite crystallization and passivates the under-coordinated Pb2+ dangling bond. PSCs fabricated with the FTO/TiO2/MAPbI(3)/Spiro-OMeTAD/Ag architecture used high quality films with less defective surfaces, present a PCE of 21.33%, retaining 91% of its initial value in ambient without any encapsulation after 30 days. These results provide insight into the surface defect passivation process achieved by halide ions balance while providing a simple and efficient process that can be extensively used to fabricate high-quality perovskite films. |
URL标识 | 查看原文 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.ciomp.ac.cn/handle/181722/64631] |
专题 | 中国科学院长春光学精密机械与物理研究所 |
推荐引用方式 GB/T 7714 | F. Y. Wang,M. F. Yang,S. Yang,X. Qu,L. L. Yang,L. Fan,J. H. Yang and F. Rosei. Iodine-assisted antisolvent engineering for stable perovskite solar cells with efficiency >21.3 %[J]. Nano Energy,2020,67:8. |
APA | F. Y. Wang,M. F. Yang,S. Yang,X. Qu,L. L. Yang,L. Fan,J. H. Yang and F. Rosei.(2020).Iodine-assisted antisolvent engineering for stable perovskite solar cells with efficiency >21.3 %.Nano Energy,67,8. |
MLA | F. Y. Wang,M. F. Yang,S. Yang,X. Qu,L. L. Yang,L. Fan,J. H. Yang and F. Rosei."Iodine-assisted antisolvent engineering for stable perovskite solar cells with efficiency >21.3 %".Nano Energy 67(2020):8. |
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