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	Effective high-order harmonic generation from metal sulfide quantum dots
	Ganeev, R. A.; Boltaev, G. S.; Kim, V. V.; Zhang, K.; Zvyagin, A. I.; Smirnov, M. S.; Ovchinnikov, O. V.; Redkin, P. V.; Wostmann, M.; Zacharias, H.
刊名	Optics Express
	2018
卷号	26期号:26页码:35013-35025
关键词	nonlinear-optical properties nanosecond clusters Optics
ISSN号	1094-4087
DOI	10.1364/oe.26.035013
英文摘要	In the past, common media for high-order harmonic generation (HHG) has been atoms and molecules. More recently, clusters, and nanoparticles have been introduced as HHG emitting media. Multi-particle media can enhance HHG yields but have more stringent requirements in determining the optimal parameters. Here, we demonstrate, for the first time, the effective application of 1-3 nm metal sulfide quantum dots (QDs) for harmonic generation in the 20 - 115 nm extreme ultraviolet range. We report on the syntheses, ablation of Ag2S, CdS, and ZnS QDs, and HHG from laser-produced plasmas by using single- and two-color pumps. We compare HHG efficiency from the ablated QDs to that of bulk metal sulfides and show a seven-fold increase in harmonic yields. Further, the study also allows us to understand the effects of QD-contained plasma spreading dynamics on HHG yield. (C) 2018 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
内容类型	期刊论文
源URL	[http://ir.ciomp.ac.cn/handle/181722/60968]
专题	中国科学院长春光学精密机械与物理研究所
推荐引用方式 GB/T 7714	Ganeev, R. A.,Boltaev, G. S.,Kim, V. V.,et al. Effective high-order harmonic generation from metal sulfide quantum dots[J]. Optics Express,2018,26(26):35013-35025.
APA	Ganeev, R. A..,Boltaev, G. S..,Kim, V. V..,Zhang, K..,Zvyagin, A. I..,...&Guo, C. L..(2018).Effective high-order harmonic generation from metal sulfide quantum dots.Optics Express,26(26),35013-35025.
MLA	Ganeev, R. A.,et al."Effective high-order harmonic generation from metal sulfide quantum dots".Optics Express 26.26(2018):35013-35025.

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