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Hollow multishell structures exercise temporal-spatial ordering and dynamic smart behaviour
Wang, Jiangyan1; Wan, Jiawei1; Yang, Nailiang1,3; Li, Quan2; Wang, Dan1,3
刊名NATURE REVIEWS CHEMISTRY
2020-02-11
页码10
DOI10.1038/s41570-020-0161-8
英文摘要A hollow multishell structure (HoMS) is an assembly of multiple shells with voids between the individual shells. Accessible through nanopores, these voids represent separate reaction environments in the same assembly, such that HoMSs have unique properties that are applicable to diverse fields. These applications have mostly exploited the large specific surface area, high loading capacity and/or buffering effect of HoMSs, benefiting the mass/energy transmission and effective surface area. In comparison, the temporal-spatial ordering of reactions, as well as the dynamic smart behaviour of HoMSs, have been less explored but are also emphasized in this Perspective. We first describe the synthesis of HoMSs and the thermodynamic and kinetic aspects of their formation. We then consider the composition and structural functionalization of each shell within a HoMS and then highlight how these enable applications based on temporal-spatial ordering and dynamic smart behaviour.
资助项目National Natural Science Foundation of China[21590795] ; National Natural Science Foundation of China[21820102002] ; National Natural Science Foundation of China[51802306] ; Scientific Instrument Developing Project of the Chinese Academy of Sciences[YZ201623]
WOS关键词METAL-ORGANIC FRAMEWORK ; DRUG-RELEASE ; MESOPOROUS ALUMINOSILICATE ; ACCURATE CONTROL ; SILICA SPHERES ; PORE STRUCTURE ; MICROSPHERES ; PH ; NANOPARTICLES ; PERFORMANCE
WOS研究方向Chemistry
语种英语
出版者NATURE PUBLISHING GROUP
WOS记录号WOS:000512843100001
资助机构National Natural Science Foundation of China ; Scientific Instrument Developing Project of the Chinese Academy of Sciences
内容类型期刊论文
源URL[http://ir.ipe.ac.cn/handle/122111/39184]  
专题中国科学院过程工程研究所
通讯作者Wang, Dan
作者单位1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing, Peoples R China
2.Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China
3.Univ Chinese Acad Sci, Beijing, Peoples R China
推荐引用方式
GB/T 7714
Wang, Jiangyan,Wan, Jiawei,Yang, Nailiang,et al. Hollow multishell structures exercise temporal-spatial ordering and dynamic smart behaviour[J]. NATURE REVIEWS CHEMISTRY,2020:10.
APA Wang, Jiangyan,Wan, Jiawei,Yang, Nailiang,Li, Quan,&Wang, Dan.(2020).Hollow multishell structures exercise temporal-spatial ordering and dynamic smart behaviour.NATURE REVIEWS CHEMISTRY,10.
MLA Wang, Jiangyan,et al."Hollow multishell structures exercise temporal-spatial ordering and dynamic smart behaviour".NATURE REVIEWS CHEMISTRY (2020):10.
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