Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites

doi:10.7503/cjcu20200461

CORC > 金属研究所 > 中国科学院金属研究所

	Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites
	Zou Run 2; Dong Xiao 2; Jiao Yilai 1; D'Agostino, Carmine 2; Yan Wenfu 3; Fan Xiaolei 2
刊名	CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE
	2021-01-10
卷号	42 期号:1 页码:74-100
关键词	Hierarchical zeolite Post-synthetic treatment Diffusion Pulsed-field gradient nuclear magnetic resonance( PFG NMR) Catalysis
ISSN号	0251-0790
DOI	10.7503/cjcu20200461
通讯作者	Fan Xiaolei(xiaolei.fan@manchester.ac.uk)
英文摘要	Hierarchical zeolites refer to zeolitic materials having bi-/multi-modal interconnective pores arranged in order of certain ranks, which improve the molecular diffusion within their frameworks, and hence the performance in their applications such as adsorption and heterogeneous catalysis. Hierarchical zeolites are commonly produced via the top-down post-synthetic treatments (such as dealumination and/or desilication) of pre-synthesized zeolites (i.e. the parent zeolites) and the bottom-up synthesis-by-design methods (such as soft/ hard templating). This review presents the recent advances (mainly post 2000) in the strategies of making hierarchical zeolites, with the emphasis on the top-down approaches due to their relatively high practicality. Since hierarchical zeolites are proposed to improve intracrystalline diffusion, experimental studies of guest molecules diffusion in hierarchical zeolites are also reviewed. Additionally, catalytic applications of hierarchical zeolites, in comparison with the conventional microporous pristine zeolites, are also commented to highlight the advantages of hierarchical zeolites to improve catalysis.
资助项目	European Union[872102] ; China Scholarship Council-The University of Manchester Joint Scholarship[201906740020] ; Programme of Introducing Talents of Discipline to Universities of China[B17020] ; National Natural Science Foundation of China[U1967215] ; National Natural Science Foundation of China[21835002] ; National Natural Science Foundation of China[21621001] ; EPSRC New Investigator Award[EP/S019138/1] ; Natural Science Foundation of Liaoning Province,China[2018010047-301] ; National Key Research and Development Program of China[SQ2019YFE011366]
WOS研究方向	Chemistry
语种	英语
出版者	HIGHER EDUCATION PRESS
WOS记录号	WOS:000607831700007
资助机构	European Union ; China Scholarship Council-The University of Manchester Joint Scholarship ; Programme of Introducing Talents of Discipline to Universities of China ; National Natural Science Foundation of China ; EPSRC New Investigator Award ; Natural Science Foundation of Liaoning Province,China ; National Key Research and Development Program of China
内容类型	期刊论文
源URL	[http://ir.imr.ac.cn/handle/321006/159029]
专题	金属研究所_中国科学院金属研究所
通讯作者	Fan Xiaolei
作者单位	1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 2.Univ Manchester, Sch Engn, Dept Chem Engn & Analyt Sci, Manchester M13 9PL, Lancs, England 3.Jilin Univ, Coll Chem, State Key Lab Inorgan Synth & Preparat Chem, Changchun 130012, Peoples R China
推荐引用方式 GB/T 7714	Zou Run,Dong Xiao,Jiao Yilai,et al. Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites[J]. CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE,2021,42(1):74-100.
APA	Zou Run,Dong Xiao,Jiao Yilai,D'Agostino, Carmine,Yan Wenfu,&Fan Xiaolei.(2021).Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites.CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE,42(1),74-100.
MLA	Zou Run,et al."Controllable Synthesis, Diffusion Study and Catalysis of Hierarchical Zeolites".CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE 42.1(2021):74-100.