Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3

doi:10.1039/d0cy00599a

CORC > 金属研究所 > 中国科学院金属研究所

	Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3
	Zheng, Kang 1; Zhou, Zhiyuan 1; Wang, Yongzhao 2; Xin, Zhiling 1; Zhao, Zhiliang 1; Zhang, Jing 1; Bo, Tingting 1; Lin, Tsungwu 3; Zhang, Bingsen 2; Shao, Lidong 1
刊名	CATALYSIS SCIENCE & TECHNOLOGY
	2020-05-21
卷号	10 期号:10 页码:3450-3457
ISSN号	2044-4753
DOI	10.1039/d0cy00599a
通讯作者	Xin, Zhiling(xinzhiling@126.com) ; Zhang, Bingsen(bszhang@imr.ac.cn) ; Shao, Lidong(lidong.shao@shiep.edu.cn)
英文摘要	We report a facile method for dispersing Mn species onto two-dimensional Co3O4 nanosheets at the nanoscale for the selective catalytic reduction (SCR) of NOx with NH3. In comparison with the reference catalysts with higher Mn loadings, the Mn/Co3O4 (0.8 wt%) catalyst exhibits improved catalytic activity and a high H2O-resistance ability. Due to the strong interaction between cobalt and manganese oxides and the increased surface area of the Co3O4 nanosheets, the catalyst with an ultralow amount of Mn at the nanoscale possesses stronger reducibility, abundant Co3+ and surface oxygen species, which in turn enhance the NH3-SCR activity.
资助项目	Science and Technology Commission of Shanghai Municipality[19DZ2271100] ; National Natural Science Foundation of China[21761132025] ; Liao Ning Revitalization Talents Program[XLYC1807175] ; Research Fund of SYNL[L2019F38]
WOS研究方向	Chemistry
语种	英语
出版者	ROYAL SOC CHEMISTRY
WOS记录号	WOS:000538156300026
资助机构	Science and Technology Commission of Shanghai Municipality ; National Natural Science Foundation of China ; Liao Ning Revitalization Talents Program ; Research Fund of SYNL
内容类型	期刊论文
源URL	[http://ir.imr.ac.cn/handle/321006/139100]
专题	金属研究所_中国科学院金属研究所
通讯作者	Xin, Zhiling; Zhang, Bingsen; Shao, Lidong
作者单位	1.Shanghai Univ Elect Power, Shanghai Key Lab Mat Protect & Adv Mat Elect Powe, 2103 Pingliang Rd, Shanghai 200090, Peoples R China 2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Peoples R China 3.Tunghai Univ, Dept Chem, 181,Sec 3,Port Rd, Taichung 40704, Taiwan
推荐引用方式 GB/T 7714	Zheng, Kang,Zhou, Zhiyuan,Wang, Yongzhao,et al. Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3[J]. CATALYSIS SCIENCE & TECHNOLOGY,2020,10(10):3450-3457.
APA	Zheng, Kang.,Zhou, Zhiyuan.,Wang, Yongzhao.,Xin, Zhiling.,Zhao, Zhiliang.,...&Shao, Lidong.(2020).Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3.CATALYSIS SCIENCE & TECHNOLOGY,10(10),3450-3457.
MLA	Zheng, Kang,et al."Ultralow loading of nanostructured Mn species onto two-dimensional Co3O4 nanosheets for selective catalytic reduction of NOx with NH3".CATALYSIS SCIENCE & TECHNOLOGY 10.10(2020):3450-3457.