Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol

doi:10.1016/j.cplett.2020.137306

CORC > 金属研究所 > 中国科学院金属研究所

	Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol
	Zhao, Zhiliang 2; Zhang, Jing 2; Wang, Yongzhao 1; Guo, Wenyao 2; Lv, Lin 2; Li, Baiyu 3; Zheng, Kang 2; Bo, Tingting 2; Peng, Dengchao 2; Zhou, Zhiyuan 2
刊名	CHEMICAL PHYSICS LETTERS
	2020-05-01
卷号	746 页码:6
关键词	Pd nanoparticles Solvent-free oxidation Benzyl alcohol Graphene oxide Aerogel
ISSN号	0009-2614
DOI	10.1016/j.cplett.2020.137306
通讯作者	Guo, Wenyao(guowenyao@shiep.edu.cn) ; Zhang, Bingsen(bszhang@imr.ac.cn) ; Shao, Lidong(lidong.shao@shiep.edu.cn)
英文摘要	In this work, Pd/reduced graphene oxide (Pd/RGO) aerogels, with large surface areas and wrinkles, are obtained through the lyophilisation, vacuum and reduction treatments. Pd/RGO aerogels exhibit higher catalytic performances and thermal stability in comparison to the reference catalyst Pd/activated carbon (Pd/AC) in the oxidation of benzyl alcohol. The surface analyses indicate that Pd/RGO aerogels possess a higher proportion of Pd2+ than the Pd/AC catalyst. Meanwhile, the oxygen-containing functional groups can modulate the interaction between palladium and the support to form active phases for the reaction. Moreover, Pd nanoparticles (PdNPs) remain well dispersed in nanoscale on the reacted Pd/RGO aerogels.
资助项目	National Natural Science Foundation of China[21773269] ; Liao Ning Revitalization Talents Program[XLYC1807175]
WOS研究方向	Chemistry ; Physics
语种	英语
出版者	ELSEVIER
WOS记录号	WOS:000522555600027
资助机构	National Natural Science Foundation of China ; Liao Ning Revitalization Talents Program
内容类型	期刊论文
源URL	[http://ir.imr.ac.cn/handle/321006/137850]
专题	金属研究所_中国科学院金属研究所
通讯作者	Guo, Wenyao; Zhang, Bingsen; Shao, Lidong
作者单位	1.Chinese Acad Sci, Shenyang Natl Lab Mat Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110016, Peoples R China 2.Shanghai Univ Elect Power, Shanghai Key Lab Mat Protect & Adv Mat Elect Powe, 2103 Pingliang Rd, Shanghai 200090, Peoples R China 3.Nantong Vocat Univ, 89 Qingnian Rd, Nantong 226006, Peoples R China
推荐引用方式 GB/T 7714	Zhao, Zhiliang,Zhang, Jing,Wang, Yongzhao,et al. Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol[J]. CHEMICAL PHYSICS LETTERS,2020,746:6.
APA	Zhao, Zhiliang.,Zhang, Jing.,Wang, Yongzhao.,Guo, Wenyao.,Lv, Lin.,...&Shao, Lidong.(2020).Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol.CHEMICAL PHYSICS LETTERS,746,6.
MLA	Zhao, Zhiliang,et al."Thermally stable Pd/reduced graphene oxide aerogel catalysts for solvent-free oxidation of benzyl alcohol".CHEMICAL PHYSICS LETTERS 746(2020):6.