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Deep eutectic solvents from hemicellulose-derived acids for the cellulosic ethanol refining of Akebia' herbal residues
Yu, Qiang1; Zhang, Aiping2; Wang, Wen1; Chen, Long1,3; Bai, Ruxue1,3; Zhuang, Xinshu1; Wang, Qiong1; Wang, Zhongming1; Yuan, Zhenhong1
刊名BIORESOURCE TECHNOLOGY
2018
卷号247页码:705-710
关键词Deep eutectic solvents Herb residues Pretreatment Enzymatic digestibility Ethanol
ISSN号0960-8524
DOI10.1016/j.biortech.2017.09.159
通讯作者Wang, Qiong(wangqiong@ms.giec.ac.cn)
英文摘要Here, the potential use of herbal residues of Akebia as feedstock for ethanol production is evaluated. Additionally, five deep eutectic solvents from hemicellulose-derived acids were prepared to overcome biomass recalcitrance. Reaction temperatures had more significant influences on solid loss and chemical composition than the molar ratios of choline chloride (ChCl) to derived acids. Glycolic acid resulted in the maximum levels of lignin, xylan and glucan removal, which were 60.0%, 100% and 71.5%, respectively, at 120 degrees C with a 1: 6 M ratio of ChCl-glycolic acid. In contrast, ChCl-formic acid resulted in the greatest level of glucan retention, at 97.8%, with a lignin removal rate of 40.7% under the same pretreatment conditions. Moreover, ChCl loading could significantly enhance the selectivity of carboxylic acid for lignin dissolution. A 98.0% level of subsequent enzymatic saccharification and a 100% ethanol yield were achieved after ChCl-formic acid pretreatments of Akebia' herbal residues.
资助项目Pearl River S & T Nova Program of Guangzhou, China[201610010110] ; Young Top-notch Talent of Guangdong Province, China[2016TQ03N647] ; National Natural Science Foundation of China[31770617] ; National Natural Science Foundation of China[21506216] ; National Natural Science Foundation of China[51506207] ; National Natural Science Foundation of China[51561145015] ; Science and Technology Planning Project of Guangdong Province, China[2014A010106023] ; Natural Science Foundation of Guangdong Province[2015A030311022] ; Natural Science Foundation for the Research Team of Guangdong Province[2016A030312007] ; Youth Innovation Promotion Association, CAS[2015289]
WOS关键词LIQUID HOT-WATER ; FLUIDIZED-BED ; ENZYMATIC DIGESTIBILITY ; PRETREATMENT ; LIGNIN ; GASIFICATION ; REMOVAL ; LIGNOCELLULOSE ; HYDROLYSIS ; PYROLYSIS
WOS研究方向Agriculture ; Biotechnology & Applied Microbiology ; Energy & Fuels
语种英语
出版者ELSEVIER SCI LTD
WOS记录号WOS:000417841800088
资助机构Pearl River S & T Nova Program of Guangzhou, China ; Young Top-notch Talent of Guangdong Province, China ; National Natural Science Foundation of China ; Science and Technology Planning Project of Guangdong Province, China ; Natural Science Foundation of Guangdong Province ; Natural Science Foundation for the Research Team of Guangdong Province ; Youth Innovation Promotion Association, CAS
内容类型期刊论文
源URL[http://ir.giec.ac.cn/handle/344007/22822]  
专题中国科学院广州能源研究所
通讯作者Wang, Qiong
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Guangdong, Peoples R China
2.South China Agr Univ, Coll Forestry & Landscape Architecture, Guangzhou 510642, Guangdong, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100039, Peoples R China
推荐引用方式
GB/T 7714
Yu, Qiang,Zhang, Aiping,Wang, Wen,et al. Deep eutectic solvents from hemicellulose-derived acids for the cellulosic ethanol refining of Akebia' herbal residues[J]. BIORESOURCE TECHNOLOGY,2018,247:705-710.
APA Yu, Qiang.,Zhang, Aiping.,Wang, Wen.,Chen, Long.,Bai, Ruxue.,...&Yuan, Zhenhong.(2018).Deep eutectic solvents from hemicellulose-derived acids for the cellulosic ethanol refining of Akebia' herbal residues.BIORESOURCE TECHNOLOGY,247,705-710.
MLA Yu, Qiang,et al."Deep eutectic solvents from hemicellulose-derived acids for the cellulosic ethanol refining of Akebia' herbal residues".BIORESOURCE TECHNOLOGY 247(2018):705-710.
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