Sources and radiocarbon ages of aerosol organic carbon along the east coast of China and implications for atmospheric fossil carbon contributions to China marginal seas

doi:10.1016/j.scitotenv.2017.11.201

CORC > 烟台海岸带研究所 > 中国科学院烟台海岸带研究所 > 中科院海岸带环境过程与生态修复重点实验室 > 近岸生态与环境实验室

	Sources and radiocarbon ages of aerosol organic carbon along the east coast of China and implications for atmospheric fossil carbon contributions to China marginal seas
	Yu, Meng ; Guo, Zhigang ; Wang, Xuchen ; Eglinton, Timothy Ian ; Yuan, Zineng ; Xing, Lei ; Zhang, Hailong ; Zhao, Meixun
刊名	SCIENCE OF THE TOTAL ENVIRONMENT
	2018-04-01
卷号	619 页码:957-965
关键词	Aerosols Radiocarbon (C-14) tracer Total organic carbon Fossil carbon China marginal seas
ISSN号	0048-9697
DOI	10.1016/j.scitotenv.2017.11.201
产权排序	[Yu, Meng ; Wang, Xuchen ; Xing, Lei ; Zhang, Hailong ; Zhao, Meixun] Ocean Univ China, Minist Educ, Key Lab Marine Chem Theory & Technol, 238 Songling Rd, Qingdao 266100, Shandong, Peoples R China ; [Yu, Meng ; Zhao, Meixun] Qingdao Natl Lab Marine Sci & Technol, Lab Marine Ecol & Environm Sci, Qingdao, Peoples R China ; [Guo, Zhigang] Fudan Univ, Shanghai Key Lab Atmospher Particle Pollut & Prev, Dept Environm Sci & Engn, Shanghai, Peoples R China ; [Eglinton, Timothy Ian] Swiss Fed Inst Technol, Dept Earth Sci, Inst Geol, CH-8092 Zurich, Switzerland ; [Yuan, Zineng] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai, Peoples R China
文献子类	Article
英文摘要	Aerosol deposition is an important mechanism for the delivery of terrestrial organic carbon (OC) to marginal seas, but OC age characteristics of aerosols are not well constrained and their contributions to sediment OC burial have not been quantified. Total suspended particle samples were collected along the east coast of China at Changdao (CD), Qingdao (QD) and Huaniao Island (HNI), and were analyzed for total organic carbon (TOC) isotopes (C-13 and C-14) in order to bridge this information gap. TOC delta C-13 and Delta C-14 values ranged from -23.6 to -30.5 parts per thousand, and -153 to -687 parts per thousand, respectively, with the latter corresponding to C-14 ages ranging from 1280 to 9260 yr. Estimated contributions of fossil carbon to TOC based on C-14 mass balance approach ranged from 26 to 73%, with strong seasonal variations in fossil carbon observed at CD. Fossil carbon at CD showed the highest proportion (73%) in winter, reflecting anthropogenic emissions and the lowest proportion (26%) in summer, caused by bio-mass contribution (annual ave., 52% +/- 17%). In contrast, the fossil carbon at both QD (57-64%) and HNI (57-67%) dominated throughout the year, reflecting local anthropogenic influences and long-range transport. Mass balance estimates indicate that atmospheric deposition and riverine export accounted for 31% and 69% of fossil carbon inputs to the China marginal seas (CMS) respectively, with fossil carbon burial efficiencies approaching 100% in the CMS. On a global scale, an atmospheric fossil carbon deposition flux of 17.2 Tg C yr(-1) was estimated, equivalent to 40% of the estimated fluvial flux to the ocean, and potentially accounting for 24-41% of fossil OC burial in marine sediments. Therefore, the atmospheric deposition constitutes an important source of fossil carbon to marine sediments, and could play a key role in regional and global scale OC budgets and biogeochemical cycles. (c) 2017 Elsevier B.V. All rights reserved.
WOS关键词	ASIAN CONTINENTAL OUTFLOW ; SOURCE APPORTIONMENT ; YELLOW SEA ; BLACK CARBON ; ANTHROPOGENIC SOURCES ; BACKGROUND SITE ; RIVER DELTA ; RURAL SITE ; BOHAI SEA ; MATTER
WOS研究方向	Environmental Sciences & Ecology
语种	英语
WOS记录号	WOS:000424144200097
资助机构	National Key Research and Development Program of China [2016YFA0601403] ; National Natural Science Foundation of China [41520104009, 41521064] ; "111" Project [B13030]
内容类型	期刊论文
源URL	[http://ir.yic.ac.cn/handle/133337/24382]
专题	烟台海岸带研究所_近岸生态与环境实验室
作者单位	1.Swiss Fed Inst Technol, Dept Earth Sci, Inst Geol, CH-8092 Zurich, Switzerland; 2.Qingdao Natl Lab Marine Sci & Technol, Lab Marine Ecol & Environm Sci, Qingdao, Peoples R China; 3.Ocean Univ China, Minist Educ, Key Lab Marine Chem Theory & Technol, 238 Songling Rd, Qingdao 266100, Shandong, Peoples R China; 4.Fudan Univ, Shanghai Key Lab Atmospher Particle Pollut & Prev, Dept Environm Sci & Engn, Shanghai, Peoples R China; 5.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai, Peoples R China
推荐引用方式 GB/T 7714	Yu, Meng,Guo, Zhigang,Wang, Xuchen,et al. Sources and radiocarbon ages of aerosol organic carbon along the east coast of China and implications for atmospheric fossil carbon contributions to China marginal seas[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2018,619:957-965.
APA	Yu, Meng.,Guo, Zhigang.,Wang, Xuchen.,Eglinton, Timothy Ian.,Yuan, Zineng.,...&Zhao, Meixun.(2018).Sources and radiocarbon ages of aerosol organic carbon along the east coast of China and implications for atmospheric fossil carbon contributions to China marginal seas.SCIENCE OF THE TOTAL ENVIRONMENT,619,957-965.
MLA	Yu, Meng,et al."Sources and radiocarbon ages of aerosol organic carbon along the east coast of China and implications for atmospheric fossil carbon contributions to China marginal seas".SCIENCE OF THE TOTAL ENVIRONMENT 619(2018):957-965.