Ammonia-Assisted Proton Transfer Reaction Mass Spectrometry for Detecting Triacetone Triperoxide (TATP) Explosive | |
Zhang, Qiangling3,4; Zou, Xue3; Liang, Qu3,4; Wang, Hongmei1; Huang, Chaoqun3; Shen, Chengyin2,3; Chu, Yannan3 | |
刊名 | JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY |
2019-03-01 | |
卷号 | 30期号:3页码:501-508 |
关键词 | Conventional PTR-MS Ammonia-assisted PTR-MS Assisted gases TATP |
ISSN号 | 1044-0305 |
DOI | 10.1007/s13361-018-2108-6 |
英文摘要 | Proton transfer reaction mass spectrometry (PTR-MS) usually detects different types of compounds by changing the discharge gas to produce different reagent ions in the ion source. In the present work, a novel method of changing reagent ions, ammonia-assisted PTR-MS, was developed. Through an injection port bypass, ammonia was injected into a homemade PTR-MS device. A conventional PTR-MS apparatus with reagent ions H3O+(H2O)(n) (n=0, 1, 2) can be converted to an ammonia-assisted PTR-MS with reagent ions NH4+.The new method was introduced to detect triacetone triperoxide (TATP) explosive material. Results showed that the sensitivity is enhanced more than 37 times compared with TATP detection using conventional PTR-MS and the limit of detection (LOD) could reach 1.3ppb. TATP in real complex matrixes can also be detected successfully using this method. Compared to conventional PTR-MS, ammonia-assisted PTR-MS has better sensitivity and better LOD for TATP detection, and the technique provides common users with a convenient and quick method to change reagent ions. The users of PTR-MS can easily obtain other reagent ions by injecting different assisted gases into an injection port to meet different detection needs. |
资助项目 | National Key R&D Program of China[2016YFC0200200] ; National Natural Science Foundation of China[21777163] ; National Natural Science Foundation of China[21477132] ; National Natural Science Foundation of China[21577145] ; Anhui Provincial Program for Science and Technology Development, China[1604d0802001] ; Key Program of 13th Five-Year Plan, CASHIPS[KP-2017-25] |
WOS关键词 | VOLATILE ORGANIC-COMPOUNDS ; ION MOBILITY SPECTROMETRY ; PTR-MS ; EXTRACTION ; SENSOR |
WOS研究方向 | Biochemistry & Molecular Biology ; Chemistry ; Spectroscopy |
语种 | 英语 |
出版者 | SPRINGER |
WOS记录号 | WOS:000461325300012 |
资助机构 | National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Anhui Provincial Program for Science and Technology Development, China ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS ; Key Program of 13th Five-Year Plan, CASHIPS |
内容类型 | 期刊论文 |
源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/42495] |
专题 | 医学物理与技术中心 合肥物质科学研究院_中科院安徽光学精密机械研究所 |
通讯作者 | Shen, Chengyin; Chu, Yannan |
作者单位 | 1.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Hefei 230031, Anhui, Peoples R China 2.Chinese Acad Sci, Hefei Canc Hosp, Hefei 230031, Anhui, Peoples R China 3.Chinese Acad Sci, Hefei Inst Phys Sci, Ctr Med Phys & Technol, Anhui Prov Key Lab Med Phys & Technol, Hefei 230031, Anhui, Peoples R China 4.Univ Sci & Technol China, Hefei 230026, Anhui, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Qiangling,Zou, Xue,Liang, Qu,et al. Ammonia-Assisted Proton Transfer Reaction Mass Spectrometry for Detecting Triacetone Triperoxide (TATP) Explosive[J]. JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY,2019,30(3):501-508. |
APA | Zhang, Qiangling.,Zou, Xue.,Liang, Qu.,Wang, Hongmei.,Huang, Chaoqun.,...&Chu, Yannan.(2019).Ammonia-Assisted Proton Transfer Reaction Mass Spectrometry for Detecting Triacetone Triperoxide (TATP) Explosive.JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY,30(3),501-508. |
MLA | Zhang, Qiangling,et al."Ammonia-Assisted Proton Transfer Reaction Mass Spectrometry for Detecting Triacetone Triperoxide (TATP) Explosive".JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY 30.3(2019):501-508. |
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