Compositional engineering of sulfides, phosphides, carbides, nitrides, oxides, and hydroxides for water splitting

doi:10.1039/d0ta05038e

	Compositional engineering of sulfides, phosphides, carbides, nitrides, oxides, and hydroxides for water splitting
	Sun, Yiqiang 2; Zhang, Tao 3; Li, Cuncheng 2; Xu, Kun 1; Li, Yue 3
刊名	JOURNAL OF MATERIALS CHEMISTRY A
	2020-07-21
卷号	8
ISSN号	2050-7488
DOI	10.1039/d0ta05038e
通讯作者	Li, Cuncheng(chm_licc@ujn.edu.cn) ; Xu, Kun(kunxu@ustc.edu.cn) ; Li, Yue(yueli@issp.ac.cn)
英文摘要	Global environmental and energy crises have attracted wide attention and led to ongoing efforts to search for sustainable energy storage and conversion systems that can meet the energy needs of modern society. Electrocatalytic water splitting driven by renewable-energy-resource-derived electricity has been identified as a potential and practical strategy for future energy generation. Exploring nonprecious-metal-based electrocatalysts with high activity and tolerance is the prerequisite for the widespread application of this energy storage model. Heteroatom-regulated electrocatalysts with controllable components as well as electronic structure have unlimited potential toward the pursuit of high-efficiency electrocatalysts and they have been recognized as the perfect platform for establishing clear structure-property relationships. Therefore, in this review, the compositional engineering of recently reported transition-metal-compound-based water-splitting catalysts with multiple anion, cation, and zero-valent-element regulations were summarized. Particular emphasis is placed on the unique role of different doping configurations for each doping type in enhancing the electrocatalytic activities and stability of heteroatom-regulated electrocatalysts by exposing the active sites, regulating the electronic structure, and promoting the electrical conductivity. Finally, some personal perspectives on the design and development of heteroatom-doped electrocatalysts are shared to indicate the possible prospective development of transition-metal-compound-based electrocatalysts.
资助项目	National Natural Science Foundation of China[51671094] ; Shandong Provincial Natural Science Foundation, China[ZR2019BEM007] ; Shandong Provincial Natural Science Foundation, China[ZR2016BM25] ; Jinan Research Leader's Studio[2019GXRC053] ; UJN ; National Science Fund for Distinguished Young Scholars[51825103] ; Natural Science Foundation of China[51771188] ; Natural Science Foundation of China[51571189] ; Open Project of State Key Laboratory of Environment-Friendly Energy Materials[19kfhg08] ; Anhui Provincial Natural Science Foundation[1708085QE92] ; Guangdong Basic and Applied Basic Research Foundation[2019A1515110231] ; Shandong Postdoctoral Innovative Talents Support Plan
WOS关键词	HYDROGEN EVOLUTION REACTION ; LAYERED DOUBLE HYDROXIDE ; EFFICIENT BIFUNCTIONAL ELECTROCATALYST ; MOS2 ULTRATHIN NANOSHEETS ; PHOSPHORUS-DOPED COS2 ; HIGHLY EFFICIENT ; HIGH-PERFORMANCE ; ACTIVE-SITES ; METAL ELECTROCATALYSTS ; ELECTRONIC-STRUCTURE
WOS研究方向	Chemistry ; Energy & Fuels ; Materials Science
语种	英语
出版者	ROYAL SOC CHEMISTRY
WOS记录号	WOS:000548452100001
资助机构	National Natural Science Foundation of China ; Shandong Provincial Natural Science Foundation, China ; Jinan Research Leader's Studio ; UJN ; National Science Fund for Distinguished Young Scholars ; Natural Science Foundation of China ; Open Project of State Key Laboratory of Environment-Friendly Energy Materials ; Anhui Provincial Natural Science Foundation ; Guangdong Basic and Applied Basic Research Foundation ; Shandong Postdoctoral Innovative Talents Support Plan
内容类型	期刊论文
源URL	[http://ir.hfcas.ac.cn:8080/handle/334002/102977]
专题	中国科学院合肥物质科学研究院
通讯作者	Li, Cuncheng; Xu, Kun; Li, Yue
作者单位	1.Anhui Univ, Dept Chem, Hefei 230601, Peoples R China 2.Univ Jinan, Sch Chem & Chem Engn, Jinan 250022, Peoples R China 3.Chinese Acad Sci, Key Lab Mat Phys, Anhui Key Lab Nanomat & Nanotechnol, Inst Solid State Phys, Hefei 230031, Peoples R China
推荐引用方式 GB/T 7714	Sun, Yiqiang,Zhang, Tao,Li, Cuncheng,et al. Compositional engineering of sulfides, phosphides, carbides, nitrides, oxides, and hydroxides for water splitting[J]. JOURNAL OF MATERIALS CHEMISTRY A,2020,8.
APA	Sun, Yiqiang,Zhang, Tao,Li, Cuncheng,Xu, Kun,&Li, Yue.(2020).Compositional engineering of sulfides, phosphides, carbides, nitrides, oxides, and hydroxides for water splitting.JOURNAL OF MATERIALS CHEMISTRY A,8.
MLA	Sun, Yiqiang,et al."Compositional engineering of sulfides, phosphides, carbides, nitrides, oxides, and hydroxides for water splitting".JOURNAL OF MATERIALS CHEMISTRY A 8(2020).