Recent Advances in Liquid-Like Thermoelectric Materials | |
Zhao, Kunpeng; Qiu, Pengfei; Shi, Xun; Chen, Lidong | |
刊名 | ADVANCED FUNCTIONAL MATERIALS |
2019-12-31 | |
关键词 | liquid-like sublattices superionic thermoelectrics transport properties |
ISSN号 | 1616-301X |
DOI | 10.1002/adfm.201903867 |
文献子类 | Review; Early Access |
英文摘要 | Thermoelectric technology has attracted great attention due to its ability to recover and convert waste heat into readily available electric energy. Among the various candidate materials, liquid-like compounds have received tremendous research interest on account of their intrinsically ultralow lattice thermal conductivity, tunable electrical properties, and high thermoelectric performance. Despite their complex phase transitions and diverse crystal structures, liquid-like materials have two independent sublattices in common: one rigid sublattice formed by immobile ions for the free transport of electrons and one liquid-like sublattice consisting of highly mobile ions to interrupt the thermal transports. This review first outlines the common structural features of liquid-like thermoelectrics, along with their unusual electron and phonon transport behaviors that well satisfy the concept of "phonon-liquid electron-crystal." Next, some commonly adopted strategies for further improving their thermoelectric performance are highlighted. The main progress achieved in the typical liquid-like TE materials is then summarized, with an emphasis on their diverse crystal structures, common characteristics, and unique transport properties. The recent understandings on the stability issue of liquid-like TE materials are also introduced. Finally, an outlook is given for the liquid-like materials with the aim to boost further development in this exciting scientific subfield. |
WOS关键词 | LOW THERMAL-CONDUCTIVITY ; X-RAY-DIFFRACTION ; PHASE-TRANSITION ; COPPER SELENIDE ; SUPERIONIC CONDUCTORS ; CHEMICAL-STABILITY ; CRYSTAL-STRUCTURE ; SINGLE-CRYSTAL ; POWER-FACTOR ; ENERGY-GAP |
WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
语种 | 英语 |
出版者 | WILEY-V C H VERLAG GMBH |
内容类型 | 期刊论文 |
源URL | [http://ir.sic.ac.cn/handle/331005/27546] |
专题 | 中国科学院上海硅酸盐研究所 |
推荐引用方式 GB/T 7714 | Zhao, Kunpeng,Qiu, Pengfei,Shi, Xun,et al. Recent Advances in Liquid-Like Thermoelectric Materials[J]. ADVANCED FUNCTIONAL MATERIALS,2019. |
APA | Zhao, Kunpeng,Qiu, Pengfei,Shi, Xun,&Chen, Lidong.(2019).Recent Advances in Liquid-Like Thermoelectric Materials.ADVANCED FUNCTIONAL MATERIALS. |
MLA | Zhao, Kunpeng,et al."Recent Advances in Liquid-Like Thermoelectric Materials".ADVANCED FUNCTIONAL MATERIALS (2019). |
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