Ambient conditions disordered-ordered phase transition of two-dimensional interfacial water molecules dependent on charge dipole moment

doi:10.1103/PhysRevMaterials.3.065602

CORC > 上海应用物理研究所 > 中国科学院上海应用物理研究所 > 中科院上海应用物理研究所2011-2017年

	Ambient conditions disordered-ordered phase transition of two-dimensional interfacial water molecules dependent on charge dipole moment
	Wang, CL ; Qi, CH ; Tu, YS ; Nie, XC ; Liang, SS
刊名	PHYSICAL REVIEW MATERIALS
	2019
卷号	3 期号:6 页码:—
关键词	CONFINED WATER HOMOGENEOUS NUCLEATION SURFACE POLARITY METAL-SURFACES ICE NUCLEATION HYDRATION LIQUID MODEL TEMPERATURE MONOLAYER
ISSN号	2475-9953
DOI	10.1103/PhysRevMaterials.3.065602
文献子类	期刊论文
英文摘要	Phase transitions of water molecules are commonly expected to occur only under extreme conditions, such as nanoconfinement, high pressure, or low temperature. We herein report the disordered-ordered phase transition of two-dimensional interfacial water molecules under ambient conditions using molecular-dynamics simulations. This phase transition is greatly dependent on the charge dipole moment, production of both charge values, and the dipole length of the solid surface. The phase transition can be identified by a sharp change in water-water interaction energies and the order parameters of the two-dimensional interfacial water monolayer, under a tiny dipole moment change near the critical dipole moment. The critical dipole moment of the solid material surface can classify a series of materials that can induce distinct ordered phases of surface water, which may also result in surface wetting, friction, and other properties.
语种	英语
内容类型	期刊论文
源URL	[http://ir.sinap.ac.cn/handle/331007/31464]
专题	上海应用物理研究所_中科院上海应用物理研究所2011-2017年
作者单位	1.Univ Nebraska, Dept Chem, Lincoln, NE 68588 USA 2.Chinese Acad Sci, Shanghai Inst Appl Phys, Div Interfacial Water, Shanghai 201800, Peoples R China; 3.Chinese Acad Sci, Shanghai Inst Appl Phys, Key Lab Interfacial Phys & Technol, Shanghai 201800, Peoples R China; 4.Chinese Acad Sci, Shanghai Adv Res Inst, Shanghai 201210, Peoples R China; 5.Shandong Univ, Sch Phys, Jinan 250100, Shandong, Peoples R China; 6.Yangzhou Univ, Coll Phys Sci & Technol, Yangzhou 225009, Jiangsu, Peoples R China;
推荐引用方式 GB/T 7714	Wang, CL,Qi, CH,Tu, YS,et al. Ambient conditions disordered-ordered phase transition of two-dimensional interfacial water molecules dependent on charge dipole moment[J]. PHYSICAL REVIEW MATERIALS,2019,3(6):—.
APA	Wang, CL,Qi, CH,Tu, YS,Nie, XC,&Liang, SS.(2019).Ambient conditions disordered-ordered phase transition of two-dimensional interfacial water molecules dependent on charge dipole moment.PHYSICAL REVIEW MATERIALS,3(6),—.
MLA	Wang, CL,et al."Ambient conditions disordered-ordered phase transition of two-dimensional interfacial water molecules dependent on charge dipole moment".PHYSICAL REVIEW MATERIALS 3.6(2019):—.