Direct Methane Conversion under Mild Condition by Thermo-, Electro-, or Photocatalysis

doi:10.1016/j.chempr.2019.05.008

	Direct Methane Conversion under Mild Condition by Thermo-, Electro-, or Photocatalysis
	Meng, Xianguang 1; Cui, Xiaoju 1,2,3; Rajan, N. Pethan 1; Yu, Liang 1,3; Deng, Dehui 1,2,3; Bao, Xinhe 1,3
刊名	CHEM
	2019-09-12
卷号	5 期号:9 页码:2296-2325
ISSN号	2451-9294
DOI	10.1016/j.chempr.2019.05.008
通讯作者	Deng, Dehui(dhdeng@dicp.ac.cn)
英文摘要	Direct conversion of earth-abundant methane into value-added chemicals under mild conditions is an attractive technology in response to the increasing industrial demand of feedstocks and worldwide appeal of energy conservation. Exploring advanced low-temperature C-H activation catalysts and reaction systems is the key to converting methane in a direct and mild manner. The recently developed reaction processes operated at low-temperature thermocatalysis systems or driven in electro- and photocatalysis systems shine light on the way to achieve efficient methane conversion with much economical energy input. In this review, we summarize the typical catalytic processes employed in these reaction systems and in particular highlight the potential heterogeneous catalysts with noteworthy C-H activation performance. We also present the progress along with our perspectives on catalyst design, theoretical simulations, the choice of reaction condition, and the method of reaction product analysis to encourage more viable technology for low-temperature methane conversion in the future.
资助项目	Ministry of Science and Technology of China[2016YFA0204100] ; Ministry of Science and Technology of China[2016YFA0200200] ; National Natural Science Foundation of China[21890753] ; National Natural Science Foundation of China[21573220] ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences (CAS)[QYZDB-SSW-JSC020] ; CAS DNL Cooperation Fund[DNL180201]
WOS关键词	DIRECT CATALYTIC CONVERSION ; LOW-TEMPERATURE OXIDATION ; ACETIC-ACID ; SELECTIVE OXIDATION ; CARBON-DIOXIDE ; MECHANISTIC INSIGHTS ; EXCHANGED ZEOLITES ; AMBIENT CONDITIONS ; NITROUS-OXIDE ; ACTIVATION
WOS研究方向	Chemistry
语种	英语
出版者	CELL PRESS
WOS记录号	WOS:000485810000008
资助机构	Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences (CAS) ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences (CAS) ; CAS DNL Cooperation Fund ; CAS DNL Cooperation Fund ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences (CAS) ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences (CAS) ; CAS DNL Cooperation Fund ; CAS DNL Cooperation Fund ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences (CAS) ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences (CAS) ; CAS DNL Cooperation Fund ; CAS DNL Cooperation Fund ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences (CAS) ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences (CAS) ; CAS DNL Cooperation Fund ; CAS DNL Cooperation Fund
内容类型	期刊论文
源URL	[http://cas-ir.dicp.ac.cn/handle/321008/173357]
专题	大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者	Deng, Dehui
作者单位	1.Chinese Acad Sci, Collaborat Innovat Ctr Chem Energy Mat, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China 2.Xiamen Univ, Coll Chem & Chem Engn, Collaborat Innovat Ctr Chem Energy Mat, State Key Lab Phys Chem Solid Surfaces, Xiamen 361005, Fujian, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100039, Peoples R China
推荐引用方式 GB/T 7714	Meng, Xianguang,Cui, Xiaoju,Rajan, N. Pethan,et al. Direct Methane Conversion under Mild Condition by Thermo-, Electro-, or Photocatalysis[J]. CHEM,2019,5(9):2296-2325.
APA	Meng, Xianguang,Cui, Xiaoju,Rajan, N. Pethan,Yu, Liang,Deng, Dehui,&Bao, Xinhe.(2019).Direct Methane Conversion under Mild Condition by Thermo-, Electro-, or Photocatalysis.CHEM,5(9),2296-2325.
MLA	Meng, Xianguang,et al."Direct Methane Conversion under Mild Condition by Thermo-, Electro-, or Photocatalysis".CHEM 5.9(2019):2296-2325.