Fast removal of ammonium ion using a hydrogel optimized with response surface methodology | |
Zheng YA(郑易安); Liu Y(刘毅); Wang AQ(王爱勤) | |
刊名 | Chemical Engineering Journal |
2011 | |
卷号 | 171期号:3页码:1201-1208 |
关键词 | Adsorption Ammonium ion Box-Behnken design Hydrogel Response surface methodology |
ISSN号 | 1385-8947 |
通讯作者 | 王爱勤 aqwang@licp.cas.cn |
中文摘要 | Response surface methodology (RSM) based on a three-level, three-variable, Box-Behnken design (BBD) was used to optimize the preparation parameters of a hydrogel consisted of polyvinyl alcohol (PVA), acrylic acid (AA) and tourmaline (Tm). With the adsorption capacity for ammonium ion (NH4+) as the response, the effects of three variables, i.e. neutralization degree (ND) of AA, ratio of PVA to AA, and ratio of Tm to AA, were investigated. The predicted appropriate preparation conditions for the hydrogel were ND of AA of 70%, PVA:AA of 0.0833 and Tm:AA of 0.5, under which a hydrogel was prepared and used as the adsorbent to remove NH4+. The effects of contact time, ion strength, NH4+ concentration, temperature, and pH value on the adsorption capacity were investigated using a batch experiment. The results indicated that the as-prepared hydrogel showed entangled three-dimensional network and had the advantages of fast adsorption rate and high adsorption capacity for NH4+ in a pH range from 3.0 to 8.0. The regeneration and reusable experiments were also performed, and it was observed that the as prepared hydrogel was stable and regenerable using strong acid (HCl) or base (NaOH) as the desorbing agents. |
学科主题 | 功能高分子 |
收录类别 | SCI |
资助信息 | 国家自然科学基金项目(20877077) |
语种 | 英语 |
WOS记录号 | WOS:000293664600052 |
公开日期 | 2012-08-30 |
内容类型 | 期刊论文 |
源URL | [http://210.77.64.217/handle/362003/81] |
专题 | 兰州化学物理研究所_环境材料与生态化学研究发展中心 |
推荐引用方式 GB/T 7714 | Zheng YA,Liu Y,Wang AQ. Fast removal of ammonium ion using a hydrogel optimized with response surface methodology[J]. Chemical Engineering Journal,2011,171(3):1201-1208. |
APA | 郑易安,刘毅,&王爱勤.(2011).Fast removal of ammonium ion using a hydrogel optimized with response surface methodology.Chemical Engineering Journal,171(3),1201-1208. |
MLA | 郑易安,et al."Fast removal of ammonium ion using a hydrogel optimized with response surface methodology".Chemical Engineering Journal 171.3(2011):1201-1208. |
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