Fast removal of ammonium ion using a hydrogel optimized with response surface methodology
Zheng YA(郑易安); Liu Y(刘毅); Wang AQ(王爱勤)
刊名Chemical Engineering Journal
2011
卷号171期号:3页码:1201-1208
关键词Adsorption Ammonium ion Box-Behnken design Hydrogel Response surface methodology
ISSN号1385-8947
通讯作者王爱勤 aqwang@licp.cas.cn
中文摘要Response surface methodology (RSM) based on a three-level, three-variable, Box-Behnken design (BBD) was used to optimize the preparation parameters of a hydrogel consisted of polyvinyl alcohol (PVA), acrylic acid (AA) and tourmaline (Tm). With the adsorption capacity for ammonium ion (NH4+) as the response, the effects of three variables, i.e. neutralization degree (ND) of AA, ratio of PVA to AA, and ratio of Tm to AA, were investigated. The predicted appropriate preparation conditions for the hydrogel were ND of AA of 70%, PVA:AA of 0.0833 and Tm:AA of 0.5, under which a hydrogel was prepared and used as the adsorbent to remove NH4+. The effects of contact time, ion strength, NH4+ concentration, temperature, and pH value on the adsorption capacity were investigated using a batch experiment. The results indicated that the as-prepared hydrogel showed entangled three-dimensional network and had the advantages of fast adsorption rate and high adsorption capacity for NH4+ in a pH range from 3.0 to 8.0. The regeneration and reusable experiments were also performed, and it was observed that the as prepared hydrogel was stable and regenerable using strong acid (HCl) or base (NaOH) as the desorbing agents.
学科主题功能高分子
收录类别SCI
资助信息国家自然科学基金项目(20877077)
语种英语
WOS记录号WOS:000293664600052
公开日期2012-08-30
内容类型期刊论文
源URL[http://210.77.64.217/handle/362003/81]  
专题兰州化学物理研究所_环境材料与生态化学研究发展中心
推荐引用方式
GB/T 7714
Zheng YA,Liu Y,Wang AQ. Fast removal of ammonium ion using a hydrogel optimized with response surface methodology[J]. Chemical Engineering Journal,2011,171(3):1201-1208.
APA 郑易安,刘毅,&王爱勤.(2011).Fast removal of ammonium ion using a hydrogel optimized with response surface methodology.Chemical Engineering Journal,171(3),1201-1208.
MLA 郑易安,et al."Fast removal of ammonium ion using a hydrogel optimized with response surface methodology".Chemical Engineering Journal 171.3(2011):1201-1208.
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