Bio-oil steam reforming, partial oxidation or oxidative steam reforming coupled with bio-oil dry reforming to eliminate CO2 emission

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	Bio-oil steam reforming, partial oxidation or oxidative steam reforming coupled with bio-oil dry reforming to eliminate CO2 emission
	Lv GX(吕功煊); Lv GX(吕功煊)
刊名	Int. J. Hydrog. Energy
	2010
卷号	35 页码:7169-7176
关键词	Steam reforming Bio-oil Carbon dioxide elimination Syngas production
ISSN号	0360-3199
通讯作者	吕功煊
中文摘要	Biomass is carbon-neutral and utilization of biomass as hydrogen resource shows no impact on atmospheric CO2 level. Nevertheless, a significant amount of CO2 is always produced in biomass gasification processes. If the CO2 produced can further react with biomass, then the biomass gasification coupled with CO2 reforming of biomass will result in a net decrease of CO2 level in atmosphere and produce the chemical raw material, syngas. To achieve this concept, a ‘‘Y’’ type reactor is developed and applied in bio-oil steam reforming, partial oxidation, or oxidative steam reforming coupled with CO2 reforming of bio-oil to eliminate the emission of CO2. The experimental results show that the reaction systems can efficiently suppress the emission of CO2 from various reforming processes. The different coupled reaction systems generate the syngas with different molar ratio of CO/H2. In addition, coke deposition is encountered in the different reforming processes. Both catalysts and experimental parameters significantly affect the coke deposition. Ni/La2O3 catalyst shows much higher resistivity toward coke deposition than Ni/Al2O3 catalyst, while employing high reaction temperature is vital for elimination of coke deposition. Although the different coupled reaction systems show different characteristic in terms of product distribution and coke deposition, which all can serve as methods for storage of the carbon from fossil fuels or air.
学科主题	环境催化与氢能
收录类别	SCI
资助信息	the 973 Project of China (2007CB613305;2009CB220003;2009AA05Z117);Solar Energy Project of Chinese Academy of Sciences (KGCX2-YW-390-1 and KGCX2-YW-390-3)
语种	英语
WOS记录号	WOS:000280601600084
公开日期	2012-09-21
内容类型	期刊论文
源URL	[http://210.77.64.217/handle/362003/466]
专题	兰州化学物理研究所_OSSO国家重点实验室兰州化学物理研究所_ERC国家工程研究中心
通讯作者	Lv GX(吕功煊); Lv GX(吕功煊)
推荐引用方式 GB/T 7714	Lv GX,Lv GX. Bio-oil steam reforming, partial oxidation or oxidative steam reforming coupled with bio-oil dry reforming to eliminate CO2 emission[J]. Int. J. Hydrog. Energy,2010,35:7169-7176.
APA	吕功煊,&吕功煊.(2010).Bio-oil steam reforming, partial oxidation or oxidative steam reforming coupled with bio-oil dry reforming to eliminate CO2 emission.Int. J. Hydrog. Energy,35,7169-7176.
MLA	吕功煊,et al."Bio-oil steam reforming, partial oxidation or oxidative steam reforming coupled with bio-oil dry reforming to eliminate CO2 emission".Int. J. Hydrog. Energy 35(2010):7169-7176.