Sources and sink of black carbon in Arctic Ocean sediments | |
Ren, Peng1; Liu, Yanguang2,3; Shi, Xuefa2; Sun, Shuwen4; Fan, Di4; Wang, Xuchen1,4 | |
刊名 | SCIENCE OF THE TOTAL ENVIRONMENT |
2019-11 | |
卷号 | 689页码:912-920 |
关键词 | Black carbon Radiocarbon Marine sediment Arctic Ocean Organic matter |
ISSN号 | 0048-9697 |
DOI | 10.1016/j.scitotenv.2019.06.437 |
英文摘要 | The concentrations and carbon isotopic (C-13, C-14) compositions of total organic carbon (TOC) and black carbon (BC) were measured for four sediment cores collected from the shelf to slope in the Arctic Ocean. Contents of TOC and BC ranged from 0.46% to 1.94% and 0.04% to 0.13% by dry weight, and BC accounted for 3.5% to 15.2% of the TOC preserved in the shelf and slope sediments. Sediment of the Chukchi shelf contained relatively high BC contents compared with the sediments of the Arctic slope, suggesting strong influence from the river and terrestrial inputs to the shelf region. Radiocarbon measurements revealed that the ages of BC are in the range of 7330 to 29,700 years (before present) and they are 4093 to 7723 years older than the C-14 ages of TOC preserved in the same sediment depths. Based on an isotopic mass balance model, we calculated that fossil fuel combustion contributed 62-96%, and biomass burning contributed 4-38% of the BC pool in the sediments of the study area. This "slow-cycling" old BC is an important fraction of the inert organic carbon pool preserved in the sediments, and represents a significant sink of atmospheric CO2 and global carbon cycle. With the thawing permafrost caused by continuous global warming, the size of this BC pool mobilized and exported by rivers to the Arctic Ocean could increase in the future. (C) 2019 Elsevier B.V. All rights reserved. |
电子版国际标准刊号 | 18791026 |
资助项目 | Marine S& T Fund of Shandong Province for Qingdao National Laboratory for Marine Science and Technology[2018SDKJ0104-3] |
WOS研究方向 | Environmental Sciences & Ecology |
语种 | 英语 |
出版者 | ELSEVIER |
WOS记录号 | WOS:000482379400088 |
内容类型 | 期刊论文 |
源URL | [http://ir.fio.com.cn:8080/handle/2SI8HI0U/30098] |
专题 | 业务部门_海洋地质与地球物理研究室 |
通讯作者 | Wang, Xuchen |
作者单位 | 1.Ocean Univ China, Inst Adv Ocean Study, Key Lab Marine Chem Theory & Technol, Qingdao, Shandong, Peoples R China 2.Minist Nat Resources, Inst Oceanog 1, Key Lab Marine Sedimentol & Environm Geol, Qingdao, Shandong, Peoples R China 3.Qingdao Natl Lab Marine Sci & Technol, Lab Marine Geol, Qingdao, Shandong, Peoples R China 4.Qingdao Natl Lab Marine Sci & Technol, Ctr Isotope Geochem & Geochronol, Qingdao, Shandong, Peoples R China |
推荐引用方式 GB/T 7714 | Ren, Peng,Liu, Yanguang,Shi, Xuefa,et al. Sources and sink of black carbon in Arctic Ocean sediments[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2019,689:912-920. |
APA | Ren, Peng,Liu, Yanguang,Shi, Xuefa,Sun, Shuwen,Fan, Di,&Wang, Xuchen.(2019).Sources and sink of black carbon in Arctic Ocean sediments.SCIENCE OF THE TOTAL ENVIRONMENT,689,912-920. |
MLA | Ren, Peng,et al."Sources and sink of black carbon in Arctic Ocean sediments".SCIENCE OF THE TOTAL ENVIRONMENT 689(2019):912-920. |
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