Polymer-Coated Graphene Aerogel Beads and Supercapacitor Application | |
Ouyang, An ; Cao, Anyuan ; Hu, Song ; Li, Yanhui ; Xu, Ruiqiao ; Wei, Jinquan ; Zhu, Hongwei ; Wu, Dehai | |
刊名 | ACS APPLIED MATERIALS & INTERFACES |
2016 | |
关键词 | graphene beads freeze casting sandwich structure composite beads supercapacitor CARBON NANOTUBES ENERGY-STORAGE OXIDE NANOCOMPOSITES ARCHITECTURES PERFORMANCE COMPOSITES ELECTRODES DEPOSITION MONOLITHS |
DOI | 10.1021/acsami.6b01965 |
英文摘要 | Graphene aerogels are highly porous materials with many energy and environmental applications; tailoring the structure and composition of pore walls within the aerogel is the key to those applications. Here, by freeze casting the graphene oxide sheets, we directly fabricated freestanding porous graphene beads containing radially oriented through channels from the sphere center to its surface. Furthermore, we introduced pseudopolymer to make reinforced, functional composite beads with a unique pore morphology. We showed that polymer layers can be coated smoothly on both sides of the pore walls, as well as on the junctions between adjacent pores, resulting in uniform polymer-graphene-polymer sandwiched structures (skeletons) throughout the bead. These composite beads significantly improved the electrochemical properties, with specific capacitances up to 669 Fig and good cyclic stability. Our results indicate that controlled fabrication of homogeneous hierarchical structures is a potential route toward high performance composite electrodes for various energy applications.; National Natural Science Foundation of China (NSFC) [51325202]; SCI(E); EI; PubMed; ARTICLE; anyuan@pku.edu.cn; 17; 11179-11187; 8 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/434196] |
专题 | 工学院 |
推荐引用方式 GB/T 7714 | Ouyang, An,Cao, Anyuan,Hu, Song,et al. Polymer-Coated Graphene Aerogel Beads and Supercapacitor Application[J]. ACS APPLIED MATERIALS & INTERFACES,2016. |
APA | Ouyang, An.,Cao, Anyuan.,Hu, Song.,Li, Yanhui.,Xu, Ruiqiao.,...&Wu, Dehai.(2016).Polymer-Coated Graphene Aerogel Beads and Supercapacitor Application.ACS APPLIED MATERIALS & INTERFACES. |
MLA | Ouyang, An,et al."Polymer-Coated Graphene Aerogel Beads and Supercapacitor Application".ACS APPLIED MATERIALS & INTERFACES (2016). |
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