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An inventory of the emission of ammonia from agricultural fertilizer application in China for 2010 and its high-resolution spatial distribution
Xu, Peng ; Zhang, Yisheng ; Gong, Weiwei ; Hou, Xikang ; Kroeze, Carolien ; Gao, Wei ; Luan, Shengji
刊名ATMOSPHERIC ENVIRONMENT
2015
关键词Ammonia Agricultural fertilizer Emission inventory Spatial and temporal patterns Uncertainty analysis SATELLITE-OBSERVATIONS ATMOSPHERIC TRANSPORT NITROGEN-OXIDES NH3 N2O AEROSOL SOUTH ASIA VOLATILIZATION DEPOSITION
DOI10.1016/j.atmosenv.2015.05.020
英文摘要In an agricultural county like China, agricultural fertilizers are the source of ammonia (NH3) emissions. However, the spatial variability in NH3 emissions is large, and the associated uncertainties affect the reliability of total NH3 emission estimates. In this study, an inventory is presented for NH3 emissions from China's agricultural fertilizer application at the city-level, and on a 1 x 1 km grid for croplands in 2010. We present NH3 emissions by source, the temporal and spatial patterns, and the associated uncertainties. The inventory is based on high-resolution activity data, regional emission factors (EFs) and related parameters that are derived from local studies. We compare our emissions estimates with previous inventories from EDGAR and other studies. The total NH3 emissions from China's agricultural fertilizer is 10.7 (8.9-12.3) TgNH(3).yr(-1). Livestock manure spreading contributes 47.5% to the total emissions, and synthetic fertilizer use by 41.9%. Rural excrement (5.0%) and cake fertilizer (5.5%) are relatively small sources. The spatial pattern of NH3 emissions from China's agricultural fertilizer were primarily concentrated in the North China Plain, the Songliao Plain, the Huaihe River Basin, the Middle-Lower Yangtze Plain, the Pearl River Delta Plain, the Sichuan Basin, the Tarim basin and the Leizhou Peninsula. Approximately 50% of the emissions are from only 76 cities. Our temporal analysis reveals a clear seasonal pattern in NH3 emissions: highest and lowest emissions are calculated for summer and winter, accounting for 42% and 14% of the total emissions, respectively. Peak emissions are calculated for July (1.7 TgNH(3).yr(-1)) and lowest emissions for January (0.5 TgNH(3).yr(-1)). The emissions are correlated with temperature, planting time and cultivation practices. (C) 2015 Elsevier Ltd. All rights reserved.; International Science AMP; Technology Cooperation Program of China [2012DFG92020]; SCI(E); EI; ARTICLE; luansj@pkusz.edu.cn; 141-148; 115
语种英语
内容类型期刊论文
源URL[http://ir.pku.edu.cn/handle/20.500.11897/417718]  
专题城市与环境学院
环境科学与工程学院
推荐引用方式
GB/T 7714
Xu, Peng,Zhang, Yisheng,Gong, Weiwei,et al. An inventory of the emission of ammonia from agricultural fertilizer application in China for 2010 and its high-resolution spatial distribution[J]. ATMOSPHERIC ENVIRONMENT,2015.
APA Xu, Peng.,Zhang, Yisheng.,Gong, Weiwei.,Hou, Xikang.,Kroeze, Carolien.,...&Luan, Shengji.(2015).An inventory of the emission of ammonia from agricultural fertilizer application in China for 2010 and its high-resolution spatial distribution.ATMOSPHERIC ENVIRONMENT.
MLA Xu, Peng,et al."An inventory of the emission of ammonia from agricultural fertilizer application in China for 2010 and its high-resolution spatial distribution".ATMOSPHERIC ENVIRONMENT (2015).
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