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Desorption behaviors of BDE-28 and BDE-47 from natural soils with different organic carbon contents
Liu, WenXin ; Cheng, FangFang ; Li, WeiBo ; Xing, BaoShan ; Tao, Shu
刊名environmental pollution
2012
关键词BDE-28 BDE-47 Soil Desorption Kinetics Isotherms POLYBROMINATED DIPHENYL ETHERS BROMINATED FLAME RETARDANTS SORPTION-DESORPTION FATE CONTAMINANTS PHENANTHRENE SEDIMENTS MATTER MECHANISMS ADSORPTION
DOI10.1016/j.envpol.2011.12.043
英文摘要Desorption kinetic and isothermal characteristics of BDE-28 and BDE-47 were investigated using natural soils with different organic carbon fractions. The results indicated that a two-compartment first-order model with dominant contribution of slow desorption could adequately describe the released kinetics of studied PBDEs. Desorption isotherms of different samples could be fitted well by linear distribution model or nonlinear Freundlich model. Moreover, most desorption procedures roughly exhibited hysteresis with respect to preceding sorption ones. At the statistically significant level of 0.05 or 0.1, total organic carbon content (f(OC)) exhibited significant correlations with the fitted parameters by the isothermal models. The correlations of f(OC) and SUM fractions (e.g., fulvic acid and humin) with the single point desorption coefficients at lower aqueous concentrations of studied PBDEs were significant; while at higher aqueous concentrations, the relationships were less significant or insignificant. Our findings may facilitate a comprehensive understanding on behaviors of PBDEs in soil systems. (C) 2012 Elsevier Ltd. All rights reserved.; http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000301395400030&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=8e1609b174ce4e31116a60747a720701 ; Environmental Sciences; SCI(E); EI; PubMed; 2; ARTICLE; 235-242; 163
语种英语
内容类型期刊论文
源URL[http://ir.pku.edu.cn/handle/20.500.11897/160628]  
专题城市与环境学院
推荐引用方式
GB/T 7714
Liu, WenXin,Cheng, FangFang,Li, WeiBo,et al. Desorption behaviors of BDE-28 and BDE-47 from natural soils with different organic carbon contents[J]. environmental pollution,2012.
APA Liu, WenXin,Cheng, FangFang,Li, WeiBo,Xing, BaoShan,&Tao, Shu.(2012).Desorption behaviors of BDE-28 and BDE-47 from natural soils with different organic carbon contents.environmental pollution.
MLA Liu, WenXin,et al."Desorption behaviors of BDE-28 and BDE-47 from natural soils with different organic carbon contents".environmental pollution (2012).
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