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One-step synthesis of ordered mesoporous CoAl2O4 spinel-based metal oxides for CO2 reforming of CH4
Xu, Leilei ; Zhang, Jian ; Wang, Fagen ; Yuan, Kaidi ; Wang, Liangjun ; Wu, Kai ; Xu, Guoqin ; Chen, Wei
刊名RSC ADVANCES
2015
关键词SUPPORTED NICKEL-CATALYSTS SOLID-SOLUTION CATALYSTS FISCHER-TROPSCH SYNTHESIS CARBON-DIOXIDE SYNTHESIS GAS BIMETALLIC CATALYSTS CO/AL2O3 CATALYSTS PARTIAL OXIDATION CO/GAMMA-AL2O3 CATALYSTS NANOCRYSTALLINE ZIRCONIA
DOI10.1039/c5ra07249b
英文摘要A series of ordered mesoporous CoAl2O4 spinel-based metal oxides with different Co content were facilely synthesized via a one-step evaporation-induced self-assembly method and utilized as catalysts for CO2 reforming of CH4. These mesoporous catalysts, which have unique textural properties and outstanding thermal stabilities, exhibited excellent catalytic performances under various reaction conditions. The ordered mesostructures in the catalysts could provide sufficiently accessible Co active sites for gaseous reactants and stabilize Co metallic nanoparticles via confinement effects within the mesoporous frameworks. These mesoporous catalysts exhibited better anti-coke abilities than non-mesoporous catalysts or traditional supported catalysts, thus acting as a promising series of potential catalyst candidates for CO2 reforming of CH4.; Singapore MOE [R143-000-542-112]; Singapore National Research Foundation CREATE-SPURc program [R-143-001-205-592]; Jiangsu Province Government Research Platform Grant and NUSRI Seed Fund; SCI(E); EI; ARTICLE; phycw@nus.edu.sg; 60; 48256-48268; 5
语种中文
内容类型期刊论文
源URL[http://ir.pku.edu.cn/handle/20.500.11897/421218]  
专题化学与分子工程学院
推荐引用方式
GB/T 7714
Xu, Leilei,Zhang, Jian,Wang, Fagen,et al. One-step synthesis of ordered mesoporous CoAl2O4 spinel-based metal oxides for CO2 reforming of CH4[J]. RSC ADVANCES,2015.
APA Xu, Leilei.,Zhang, Jian.,Wang, Fagen.,Yuan, Kaidi.,Wang, Liangjun.,...&Chen, Wei.(2015).One-step synthesis of ordered mesoporous CoAl2O4 spinel-based metal oxides for CO2 reforming of CH4.RSC ADVANCES.
MLA Xu, Leilei,et al."One-step synthesis of ordered mesoporous CoAl2O4 spinel-based metal oxides for CO2 reforming of CH4".RSC ADVANCES (2015).
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