One-step synthesis of ordered mesoporous CoAl2O4 spinel-based metal oxides for CO2 reforming of CH4 | |
Xu, Leilei ; Zhang, Jian ; Wang, Fagen ; Yuan, Kaidi ; Wang, Liangjun ; Wu, Kai ; Xu, Guoqin ; Chen, Wei | |
刊名 | RSC ADVANCES |
2015 | |
关键词 | SUPPORTED NICKEL-CATALYSTS SOLID-SOLUTION CATALYSTS FISCHER-TROPSCH SYNTHESIS CARBON-DIOXIDE SYNTHESIS GAS BIMETALLIC CATALYSTS CO/AL2O3 CATALYSTS PARTIAL OXIDATION CO/GAMMA-AL2O3 CATALYSTS NANOCRYSTALLINE ZIRCONIA |
DOI | 10.1039/c5ra07249b |
英文摘要 | A series of ordered mesoporous CoAl2O4 spinel-based metal oxides with different Co content were facilely synthesized via a one-step evaporation-induced self-assembly method and utilized as catalysts for CO2 reforming of CH4. These mesoporous catalysts, which have unique textural properties and outstanding thermal stabilities, exhibited excellent catalytic performances under various reaction conditions. The ordered mesostructures in the catalysts could provide sufficiently accessible Co active sites for gaseous reactants and stabilize Co metallic nanoparticles via confinement effects within the mesoporous frameworks. These mesoporous catalysts exhibited better anti-coke abilities than non-mesoporous catalysts or traditional supported catalysts, thus acting as a promising series of potential catalyst candidates for CO2 reforming of CH4.; Singapore MOE [R143-000-542-112]; Singapore National Research Foundation CREATE-SPURc program [R-143-001-205-592]; Jiangsu Province Government Research Platform Grant and NUSRI Seed Fund; SCI(E); EI; ARTICLE; phycw@nus.edu.sg; 60; 48256-48268; 5 |
语种 | 中文 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/421218] |
专题 | 化学与分子工程学院 |
推荐引用方式 GB/T 7714 | Xu, Leilei,Zhang, Jian,Wang, Fagen,et al. One-step synthesis of ordered mesoporous CoAl2O4 spinel-based metal oxides for CO2 reforming of CH4[J]. RSC ADVANCES,2015. |
APA | Xu, Leilei.,Zhang, Jian.,Wang, Fagen.,Yuan, Kaidi.,Wang, Liangjun.,...&Chen, Wei.(2015).One-step synthesis of ordered mesoporous CoAl2O4 spinel-based metal oxides for CO2 reforming of CH4.RSC ADVANCES. |
MLA | Xu, Leilei,et al."One-step synthesis of ordered mesoporous CoAl2O4 spinel-based metal oxides for CO2 reforming of CH4".RSC ADVANCES (2015). |
个性服务 |
查看访问统计 |
相关权益政策 |
暂无数据 |
收藏/分享 |
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。
修改评论