Controllable and large-scale fabrication of flexible ITO-free electrochromic devices by crackle pattern technology | |
Xu, ZJ; Li, WF; Huang, JN; Liu, Q; Guo, X2; Guo, WX; Liu, XY | |
刊名 | JOURNAL OF MATERIALS CHEMISTRY A |
2018-10-28 | |
卷号 | 6期号:40页码:19584-19589 |
ISSN号 | 2050-7488 |
DOI | 10.1039/c8ta07154c |
英文摘要 | Electrochromic devices (ECDs) presenting reversible color variation are considered as the most promising alternative to traditional smart windows. However, the fabrication of large-scale ECDs with high flexibility and stability is still challenging. In this work, we present a crackle pattern technology for controllable and large-scale fabrication of rectangular Ag network films for indium tin oxide-free (ITO-free) flexible ECDs. This rectangular Ag film exhibits superior mechanical robustness and controllable optoelectronic performance (2.0 sq(-1) at 91% transmittance). In the application of WO3 based ECD, the rectangular film presents an ultrafast switching time (0.25/0.18 s for bleaching/coloring) and is thus applicable in flexible displays. Moreover, this device demonstrates a large optical modulation of 76% at 630 nm and sustains 78.9% of its initial modulation even after 20000 cycles, which is close to the commercial standard for rigid ECDs. The obtained rectangular Ag films are successfully assembled into a flexible all-solid-state ECD (21 x 13 cm(2)), which can be utilized in smart windows, glasses and other fields that require bending or cutting. |
学科主题 | Chemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary |
语种 | 英语 |
WOS记录号 | WOS:000448413100030 |
内容类型 | 期刊论文 |
源URL | [http://ir.imr.ac.cn/handle/321006/79885] |
专题 | 金属研究所_中国科学院金属研究所 |
作者单位 | 1.Xiamen Univ, Fujian Prov Key Lab Soft Funct Mat Res, Res Inst Soft Matter & Biomimet, Coll Phys,Coll Mat, Xiamen 361005, Peoples R China 2.Natl Univ Singapore, Fac Sci, Dept Phys, Singapore 117542, Singapore 3.Chinese Acad Sci, Inst Met Res, Shenyang 110016, Liaoning, Peoples R China |
推荐引用方式 GB/T 7714 | Xu, ZJ,Li, WF,Huang, JN,et al. Controllable and large-scale fabrication of flexible ITO-free electrochromic devices by crackle pattern technology[J]. JOURNAL OF MATERIALS CHEMISTRY A,2018,6(40):19584-19589. |
APA | Xu, ZJ.,Li, WF.,Huang, JN.,Liu, Q.,Guo, X.,...&Liu, XY.(2018).Controllable and large-scale fabrication of flexible ITO-free electrochromic devices by crackle pattern technology.JOURNAL OF MATERIALS CHEMISTRY A,6(40),19584-19589. |
MLA | Xu, ZJ,et al."Controllable and large-scale fabrication of flexible ITO-free electrochromic devices by crackle pattern technology".JOURNAL OF MATERIALS CHEMISTRY A 6.40(2018):19584-19589. |
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