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Improving the photocatalytic activity of graphitic carbon nitride by thermal treatment in a high-pressure hydrogen atmosphere
Kang, XD; Kang, YY; Hong, XX; Sun, ZH; Zhen, C; Hu, CH; Liu, G2; Cheng, HM
刊名PROGRESS IN NATURAL SCIENCE-MATERIALS INTERNATIONAL
2018-04-01
卷号28期号:2页码:183-188
关键词Photocatalysis Carbon nitride High pressure Hydrogenation Visible light
ISSN号1002-0071
DOI10.1016/j.pnsc.2018.02.006
英文摘要Extending visible light absorption range and suppressing the recombination of photogenerated charge carriers are always important topics in developing efficient solar-driven photocatalysts. In this study, the thermal treatment process at 400 degrees C in a high-pressure hydrogen atmosphere was applied to modify graphitic carbon nitride. Compared to the normal atmospheric hydrogen treatment process, this process has the merit of producing nitrogen deficient graphitic carbon nitride in high-yield. The optimal photocatalytic activity of modified graphitic carbon nitride was demonstrated by controlling the treatment duration in the hydrogen atmosphere. The changes in the crystal structure, microstructure and optical properties of carbon nitrides were investigated by several characterizations. The relationship between the photocatalytic activity and structures of graphitic carbon nitride was preliminarily established. The results obtained in this study could provide some new ways of improving the activity of graphitic carbon nitride based photocatalyst.
学科主题Materials Science, Multidisciplinary ; Multidisciplinary Sciences
语种英语
WOS记录号WOS:000432437500010
内容类型期刊论文
源URL[http://ir.imr.ac.cn/handle/321006/80217]  
专题金属研究所_中国科学院金属研究所
作者单位1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Liaoning, Peoples R China
2.Guilin Univ Elect Technol, Guangxi Key Lab Informat Mat, Guilin 541004, Peoples R China
3.Univ Sci & Technol China, Sch Mat Sci & Engn, 72 Wenhua Rd, Shenyang 110016, Liaoning, Peoples R China
4.Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Low Dimens Mat & Device Lab, 1001 Xueyuan Rd, Shenzhen 518055, Peoples R China
5.King Abdulaziz Univ, Ctr Excellence Environm Studies, Jeddah 21589, Saudi Arabia
推荐引用方式
GB/T 7714
Kang, XD,Kang, YY,Hong, XX,et al. Improving the photocatalytic activity of graphitic carbon nitride by thermal treatment in a high-pressure hydrogen atmosphere[J]. PROGRESS IN NATURAL SCIENCE-MATERIALS INTERNATIONAL,2018,28(2):183-188.
APA Kang, XD.,Kang, YY.,Hong, XX.,Sun, ZH.,Zhen, C.,...&Cheng, HM.(2018).Improving the photocatalytic activity of graphitic carbon nitride by thermal treatment in a high-pressure hydrogen atmosphere.PROGRESS IN NATURAL SCIENCE-MATERIALS INTERNATIONAL,28(2),183-188.
MLA Kang, XD,et al."Improving the photocatalytic activity of graphitic carbon nitride by thermal treatment in a high-pressure hydrogen atmosphere".PROGRESS IN NATURAL SCIENCE-MATERIALS INTERNATIONAL 28.2(2018):183-188.
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