Distribution, pollution status, and source apportionment of trace metals in lake sediments under the influence of the South-to-North Water Transfer Project, China | |
Zhuang, Wen1,2,3; Ying, Samantha C.2; Frie, Alexander L.2; Wang, Qian3; Song, Jinming1; Liu, Yongxia3; Chen, Qing4; Lai, Xiaoying5 | |
刊名 | SCIENCE OF THE TOTAL ENVIRONMENT |
2019-06-25 | |
卷号 | 671页码:108-118 |
关键词 | Trace metals Sediment pollution Source apportionment Water transfer project Nansihu Lake |
ISSN号 | 0048-9697 |
DOI | 10.1016/j.scitotenv.2019.03.306 |
通讯作者 | Zhuang, Wen(wzhuang@yic.ac.cn) |
英文摘要 | In an effort to combat the threat of drought, China constructed the South-to-North Water Transfer Project (SNWTP), the biggest water transfer project in terms of volume with the largest beneficiary population in the world. Reports have shown that massive water diversion projects have had detrimental environmental consequences including water quality decline and freshwater habitat degradation. However, few reports have assessed the impact of the transfer project on sediment quality, which is highly susceptible to allogenic and local anthropogenic pollution. We examined the distribution characteristics of Cd, Cr, Cu, Ni, Pb and Zn in surface sediment of the largest reservoir along the East Route of SNWTP, Nansihu Lake, followed by positive matrix factorization (PMF) to determine their potential sources. We utilized enrichment factor, multiple sediment quality guidelines (SQGs), and potential ecological risk index (RI) to determine metal accumulation or pollution risk. The results show the mean concentrations of Cr, Cu, Pb, Zn were slightly lower than in samples collected in 2003, 2010 and 2012, while the mean concentrations of Cr and Ni were significantly higher than samples from previous years. Among the six metals, Cr, Cu and Ni are of higher ecological risk according to SQGs; but Cd is of higher ecological risk according to RI. PMF analysis shows that industrial production and shipping are important sources of Cr, Cu, and Ni. PMF analysis also shows that a considerable amount of trace metals, especially Cd, Cr, Pb and Zn, mainly comes from the use of pesticide fertilizers and biomass sources in farmland, and may partly enter Nansihu Lake from SNWTP. This study reveals the possible sources of trace metals to the Nansihu Lake which is part of SNWTP; the results of the study may serve as a reference for better understanding the impact of future water diversion projects on metals distribution. (C) 2019 Elsevier B.V. All rights reserved. |
资助项目 | Natural Science Foundation of Shandong Province, China[ZR2017QD012] ; Natural Science Foundation of Shandong Province, China[ZR2014DP005] ; Natural Science Foundation of Shandong Province, China[ZR2016CB29] ; National Natural Science Foundation of China[31600080] ; USDA NIFA Hatch Fund |
WOS研究方向 | Environmental Sciences & Ecology |
语种 | 英语 |
出版者 | ELSEVIER SCIENCE BV |
WOS记录号 | WOS:000466090500013 |
内容类型 | 期刊论文 |
源URL | [http://ir.qdio.ac.cn/handle/337002/157033] |
专题 | 海洋研究所_海洋生态与环境科学重点实验室 |
通讯作者 | Zhuang, Wen |
作者单位 | 1.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Ecol & Environm Sci, 7 Nanhai Rd, Qingdao 266071, Shandong, Peoples R China 2.Univ Calif Riverside, Dept Environm Sci, Riverside, CA 92521 USA 3.Zaozhuang Univ, Coll City & Architecture Engn, Zaozhuang 277160, Shandong, Peoples R China 4.Zaozhuang Univ, Coll Life Sci, Zaozhuang 277160, Shandong, Peoples R China 5.Wuhan Inst Technol, Natl Engn & Technol Res Ctr Dev & Utilizat Phosph, Wuhai 430073, Hubei, Peoples R China |
推荐引用方式 GB/T 7714 | Zhuang, Wen,Ying, Samantha C.,Frie, Alexander L.,et al. Distribution, pollution status, and source apportionment of trace metals in lake sediments under the influence of the South-to-North Water Transfer Project, China[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2019,671:108-118. |
APA | Zhuang, Wen.,Ying, Samantha C..,Frie, Alexander L..,Wang, Qian.,Song, Jinming.,...&Lai, Xiaoying.(2019).Distribution, pollution status, and source apportionment of trace metals in lake sediments under the influence of the South-to-North Water Transfer Project, China.SCIENCE OF THE TOTAL ENVIRONMENT,671,108-118. |
MLA | Zhuang, Wen,et al."Distribution, pollution status, and source apportionment of trace metals in lake sediments under the influence of the South-to-North Water Transfer Project, China".SCIENCE OF THE TOTAL ENVIRONMENT 671(2019):108-118. |
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