A Highly Efficient Sandwich-Like Symmetrical Dual-Phase Oxygen-Transporting Membrane Reactor for Hydrogen Production by Water Splitting

doi:10.1002/anie.201603528

	A Highly Efficient Sandwich-Like Symmetrical Dual-Phase Oxygen-Transporting Membrane Reactor for Hydrogen Production by Water Splitting
	Zhu, Xuefeng 2; Fang, Wei 1; Steinbach, Frank 1; Cao, Zhongwei 2; Feldhoff, Armin 1
刊名	ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
	2016-07-18
卷号	55 期号:30 页码:8648-8651
关键词	Catalyst Regeneration Hydrogen Production Membrane Reactor Methane Water Splitting
ISSN号	1433-7851
DOI	10.1002/anie.201603528
文献子类	Article
英文摘要	Water splitting coupled with partial oxidation of methane (POM) using an oxygen-transporting membrane (OTM) would be a potentially ideal way to produce high-purity hydrogen as well as syngas. Over the past decades, substantial efforts have been devoted to the development of supported membranes with appropriate configurations to achieve considerable performance improvements. Herein, we describe the design of a novel symmetrical membrane reactor with a sandwich-like structure, whereby a largescale production (>10 mL min(-1) cm(-2)) of hydrogen and syngas can be obtained simultaneously on opposite sides of the OTM. Furthermore, this special membrane reactor could regenerate the coke-deactivated catalyst in situ by water steam in a single unit. These results represent an important first step in the development of membrane separation technologies for the integration of multiple chemical processes.
WOS关键词	HOLLOW-FIBER MEMBRANES ; OXIDE FUEL-CELLS ; PARTIAL OXIDATION ; PERMEABLE MEMBRANES ; CERAMIC MEMBRANES ; SYNTHESIS GAS ; METHANE ; PERMEATION ; PERFORMANCE ; SEPARATION
WOS研究方向	Chemistry
语种	英语
出版者	WILEY-V C H VERLAG GMBH
WOS记录号	WOS:000383253500028
内容类型	期刊论文
源URL	[http://cas-ir.dicp.ac.cn/handle/321008/170206]
专题	大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者	Zhu, Xuefeng; Fang, Wei; Feldhoff, Armin
作者单位	1.Leibniz Univ Hannover, Inst Phys Chem & Electrochem, Callinstr 3A, D-30167 Hannover, Germany 2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, 457 Zhongshan Rd, Dalian 116023, Peoples R China
推荐引用方式 GB/T 7714	Zhu, Xuefeng,Fang, Wei,Steinbach, Frank,et al. A Highly Efficient Sandwich-Like Symmetrical Dual-Phase Oxygen-Transporting Membrane Reactor for Hydrogen Production by Water Splitting[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2016,55(30):8648-8651.
APA	Zhu, Xuefeng,Fang, Wei,Steinbach, Frank,Cao, Zhongwei,&Feldhoff, Armin.(2016).A Highly Efficient Sandwich-Like Symmetrical Dual-Phase Oxygen-Transporting Membrane Reactor for Hydrogen Production by Water Splitting.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,55(30),8648-8651.
MLA	Zhu, Xuefeng,et al."A Highly Efficient Sandwich-Like Symmetrical Dual-Phase Oxygen-Transporting Membrane Reactor for Hydrogen Production by Water Splitting".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 55.30(2016):8648-8651.