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	Preliminary investigation of the degradation mechanism of o, m and p-cresol using sludge-derived carbon nanosheets by catalytic oxidation based on quantum chemistry
	Ma, Lei1; Jin, Chengyu2,3; An, Luyang4; Huang, Long1; Li, Linjun1; Jin, Haibo1; Liang, Bo1; Wei, Huangzhao2; Sun, Chenglin2
刊名	Catalysis communications
	2019-02-01
卷号	120页码:59-65
关键词	Advanced oxidation Sludge-derived carbon nanosheets Quantum chemical calculation Cresols
ISSN号	1566-7367
DOI	10.1016/j.catcom.2018.11.012
通讯作者	Wei, huangzhao(whzhdicpwtg@dicp.ac.cn) ; Sun, chenglin(clsun@dicp.ac.cn)
英文摘要	Advanced oxidation technology is widely used to oxidize organic compounds in the liquid phase by oh conventionally. here, we prepared a sludge-derived carbon nanosheets, which was applied in the catalytic wet air oxidation (cwao), catalytic wet peroxide oxidation (cwpo) and catalytic wet ozone oxidation (cwoo) systems. because of its abundant oxygen-containing functional groups, the catalytic activity of nanosheets was much higher than some conventional catalysts. it was found that the first-order reaction model did not have similar characteristics as expected. combining with molecular descriptors calculated by the dft method and pls analysis, we try to explain this phenomenon for the first time and proposed possible mechanisms for the three advanced oxidation technologies.
WOS关键词	WET PEROXIDE OXIDATION ; AIR OXIDATION ; ELECTROCHEMICAL DEGRADATION ; WASTE-WATER ; TEMPERATURE ; PHENOL ; ADSORPTION ; KINETICS ; XPS
WOS研究方向	Chemistry
WOS类目	Chemistry, Physical
语种	英语
出版者	ELSEVIER SCIENCE BV
WOS记录号	WOS:000458222300013
内容类型	期刊论文
URI标识	http://www.corc.org.cn/handle/1471x/2372811
专题	大连化学物理研究所
通讯作者	Wei, Huangzhao; Sun, Chenglin
作者单位	1.Beijing Inst Petrochem Technol, Beijing Key Lab Fuels Cleaning & Adv Catalyt Emis, Coll Chem Engn, Beijing 102617, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 4.Sinosteel Anshan Res Inst Thermoenergy Co Ltd, Natl Engn Res Ctr Coking Technol, Anshan 114044, Peoples R China
推荐引用方式 GB/T 7714	Ma, Lei,Jin, Chengyu,An, Luyang,et al. Preliminary investigation of the degradation mechanism of o, m and p-cresol using sludge-derived carbon nanosheets by catalytic oxidation based on quantum chemistry[J]. Catalysis communications,2019,120:59-65.
APA	Ma, Lei.,Jin, Chengyu.,An, Luyang.,Huang, Long.,Li, Linjun.,...&Sun, Chenglin.(2019).Preliminary investigation of the degradation mechanism of o, m and p-cresol using sludge-derived carbon nanosheets by catalytic oxidation based on quantum chemistry.Catalysis communications,120,59-65.
MLA	Ma, Lei,et al."Preliminary investigation of the degradation mechanism of o, m and p-cresol using sludge-derived carbon nanosheets by catalytic oxidation based on quantum chemistry".Catalysis communications 120(2019):59-65.

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