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Highlights of major progress on single-atom catalysis in 2017
Guo, Yalin1,2; Lang, Rui1; Qiao, Botao1
刊名Catalysts
2019-02-01
卷号9期号:2页码:12
关键词Single-atom catalysis Catalyst fabrication C1 chemical conversion Strong metal-support interaction Reaction mechanism
ISSN号2073-4344
DOI10.3390/catal9020135
通讯作者Qiao, botao(bqiao@dicp.ac.cn)
英文摘要Single-atom catalysis has rapidly progressed during the last few years. in 2017, single-atom catalysts (sacs) were fabricated with higher metal loadings and designed into more delicate structures. sacs also found wide applications in c1 chemical conversion, such as selective oxidation of methane and conversion of carbon dioxide. both experimental characterizations and computational modeling revealed the presence of tunable interactions between single atom species and their surrounding chemical environment, and thus sacs may be more effective and more stable than their nanoparticle counterparts. in this mini-review, we summarize the major achievements of sacs into three main aspects: (a) the advanced synthetic methodologies, (b) catalytic performance in c1 chemistry, and (c) strong metal-support interaction induced unexpected durability. these accomplishments will shed new light on the recognition of single-atom catalysis and encourage more efforts to explore potential applications of sacs.
WOS关键词OXYGEN REDUCTION REACTION ; METAL-ORGANIC FRAMEWORKS ; FE-N-C ; SELECTIVE HYDROGENATION ; PHOTOCATALYTIC DEGRADATION ; EFFICIENT ELECTROCATALYST ; PLATINUM CATALYSTS ; ACTIVE-SITES ; OXIDATION ; CARBON
WOS研究方向Chemistry
WOS类目Chemistry, Physical
语种英语
出版者MDPI
WOS记录号WOS:000460702200029
内容类型期刊论文
URI标识http://www.corc.org.cn/handle/1471x/2372681
专题大连化学物理研究所
通讯作者Qiao, Botao
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Guo, Yalin,Lang, Rui,Qiao, Botao. Highlights of major progress on single-atom catalysis in 2017[J]. Catalysts,2019,9(2):12.
APA Guo, Yalin,Lang, Rui,&Qiao, Botao.(2019).Highlights of major progress on single-atom catalysis in 2017.Catalysts,9(2),12.
MLA Guo, Yalin,et al."Highlights of major progress on single-atom catalysis in 2017".Catalysts 9.2(2019):12.
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