Selectivity of solid phase extraction for dissolved organic matter in the hypersaline Da Qaidam Lake, China

CORC > 青海盐湖研究所 > 中国科学院青海盐湖研究所 > 青海盐湖研究所知识仓储

	Selectivity of solid phase extraction for dissolved organic matter in the hypersaline Da Qaidam Lake, China
	Yang, Keli 1,2; Zhang, Yaoling 1; Dong, Yaping 1; Li, Wu 1
刊名	ENVIRONMENTAL SCIENCE-PROCESSES & IMPACTS
	2017-11-01
卷号	19 期号:11 页码:1374-1386
文献子类	Article
英文摘要	Dissolved organic matter (DOM) was isolated from the hypersaline Da Qaidam Lake using solid-phase extraction (SPE) methods with five different adsorbents: ENVI-Carb (non-porous graphitized carbon), HLB, PPL, and XAD-8 (polymer based), and ENVI-18 (silica based). Structure-selective assessments of SPE-DOM isolated using the different adsorbents were conducted using a combination of complementary analysis techniques, including dissolved organic carbon (DOC) and dissolved organic nitrogen (DON) analysis, as well as elemental analysis, Fourier transformed infrared spectroscopy (FTIR), H-1 nuclear magnetic resonance (H-1 NMR) and pyrolysis-gas chromatography-mass spectrometry (Py-GC/MS). The results indicated that the modified polymer based adsorbents (PPL and HLB) exhibited higher DOC recoveries than the others. The PPL and ENVI-Carb cartridges can recover representative nitrogen-containing organic components from the hypersaline lake. The SPE-DOM isolates obtained using ENVI-18 and XAD-8 adsorbents contained higher proportions of purely aliphatic, alkene, and aromatic compounds; the ENVI-Carb and PPL adsorbents showed higher affinity for polar functionalized aliphatic and nitrogen-containing compounds; HLB isolate was enriched with oxygen-rich organic compounds and sulphur-bearing components. The structural and compositional features of SPE-DOM from the hypersaline Da Qaidam Lake indicated the predominately autochthonous sources of organic matter in the lake.
WOS关键词	RESONANCE MASS-SPECTROMETRY ; AQUATIC FULVIC-ACIDS ; TMAH-PY-GC/MS ; GAS CHROMATOGRAPHY/MASS SPECTROMETRY ; TETRAMETHYLAMMONIUM HYDROXIDE TMAH ; PYROLYSIS-GC-MS ; HUMIC SUBSTANCES ; CHEMICAL-CHARACTERIZATION ; FRESH-WATER ; ELEMENTAL COMPOSITION
WOS研究方向	Chemistry ; Environmental Sciences & Ecology
语种	英语
WOS记录号	WOS:000415331100002
内容类型	期刊论文
源URL	[http://ir.isl.ac.cn/handle/363002/6278]
专题	青海盐湖研究所_青海盐湖研究所知识仓储青海盐湖研究所_盐湖资源综合利用工程技术中心
作者单位	1.Chinese Acad Sci, Qinghai Inst Salt Lakes, Key Lab Comprehens & Highly Efficient Utilizat Sa, Xining 810008, Qinghai, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式 GB/T 7714	Yang, Keli,Zhang, Yaoling,Dong, Yaping,et al. Selectivity of solid phase extraction for dissolved organic matter in the hypersaline Da Qaidam Lake, China[J]. ENVIRONMENTAL SCIENCE-PROCESSES & IMPACTS,2017,19(11):1374-1386.
APA	Yang, Keli,Zhang, Yaoling,Dong, Yaping,&Li, Wu.(2017).Selectivity of solid phase extraction for dissolved organic matter in the hypersaline Da Qaidam Lake, China.ENVIRONMENTAL SCIENCE-PROCESSES & IMPACTS,19(11),1374-1386.
MLA	Yang, Keli,et al."Selectivity of solid phase extraction for dissolved organic matter in the hypersaline Da Qaidam Lake, China".ENVIRONMENTAL SCIENCE-PROCESSES & IMPACTS 19.11(2017):1374-1386.