Removal of I- from Aqueous Solutions Using a Biomass Carbonaceous Aerogel Modified with KH-560

CORC > 青海盐湖研究所 > 中国科学院青海盐湖研究所 > 青海盐湖研究所知识仓储

	Removal of I- from Aqueous Solutions Using a Biomass Carbonaceous Aerogel Modified with KH-560
	Sun, Li 1,2,3,4,5; Zhang, Yujie 3,4; Ye, Xiushen 1,2; Liu, Haining 1,2; Zhang, Huifang 1,2; Wu, Aiguo 3,4; Wu, Zhijian 1,2
刊名	ACS SUSTAINABLE CHEMISTRY & ENGINEERING
	2017-09-01
卷号	5 期号:9 页码:7700-7708
关键词	Iodide Ion Biomass Carbonaceous Aerogel Kh-560 Adsorption Regeneration
文献子类	Article
英文摘要	Materials capable of separating and removing iodine ions (I-) from aqueous solutions are significant to our society, especially human health. Adsorption is one of the effective I- separation methods. In this work, a novel biomass carbonaceous aerogel (CA) modified with 3-glycidyl-oxypropyl-trimethoxy-silane (KH-560) was prepared and used for I- adsorption for the first time. This preparation process of CA@KH-560 is easily accessible. The results of characterization demonstrated that CA and CA@KH-560 have three-dimensional porous structure with the sheetlike skeletons connected to each other, and KH-560 effectively entered into the matrix of CA. Adsorption experiments were carried out systematically by changing the pH, adsorption time, ionic strength, temperature, and ion concentration. The maximal adsorption capacity for I- is 2.5 mmol/g at an initial pH of 1.5. The adsorption can reach equilibrium within 24 h, and the data of adsorption kinetics fitted the pseudo-second-order model very well. The adsorption isotherm model Langmuir, Freundlich, and Tempkin isotherms were studied, and the results showed that the Langmuir model is the best-fitting one for the experimental results. Moreover, CA@KH-560 shows excellent regenerating ability, and the regeneration process is relatively simple.
WOS关键词	IODIDE ADSORPTION ; HIGHLY EFFICIENT ; MAGNETIC NANOMATERIAL ; GRAPHENE AEROGELS ; ACTIVATED CARBON ; ADSORBENT ; WATER ; NANOPARTICLES ; COMPOSITES ; HYDROGELS
WOS研究方向	Chemistry ; Engineering
语种	英语
WOS记录号	WOS:000410006200029
内容类型	期刊论文
源URL	[http://ir.isl.ac.cn/handle/363002/6252]
专题	青海盐湖研究所_青海盐湖研究所知识仓储青海盐湖研究所_盐湖资源与化学实验室
作者单位	1.Chinese Acad Sci, Qinghai Inst Salt Lakes, CAS Key Lab Comprehens & Highly Efficient Utiliza, 18 Xinning Rd, Xining 810008, Qinghai, Peoples R China 2.Chinese Acad Sci, Qinghai Inst Salt Lakes, Key Lab Salt Lake Resources Chem Qinghai Prov, 18 Xinning Rd, Xining 810008, Qinghai, Peoples R China 3.Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Key Lab Addit Mfg Mat Zhejiang Prov, CAS Key Lab Magnet Mat & Devices, 1219 Zhongguan West Rd, Ningbo 315201, Zhejiang, Peoples R China 4.Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Div Funct Mat & Nanodevices, 1219 Zhongguan West Rd, Ningbo 315201, Zhejiang, Peoples R China 5.Univ Chinese Acad Sci, 19 A Yuquan Rd, Beijing 100049, Peoples R China
推荐引用方式 GB/T 7714	Sun, Li,Zhang, Yujie,Ye, Xiushen,et al. Removal of I- from Aqueous Solutions Using a Biomass Carbonaceous Aerogel Modified with KH-560[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2017,5(9):7700-7708.
APA	Sun, Li.,Zhang, Yujie.,Ye, Xiushen.,Liu, Haining.,Zhang, Huifang.,...&Wu, Zhijian.(2017).Removal of I- from Aqueous Solutions Using a Biomass Carbonaceous Aerogel Modified with KH-560.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,5(9),7700-7708.
MLA	Sun, Li,et al."Removal of I- from Aqueous Solutions Using a Biomass Carbonaceous Aerogel Modified with KH-560".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 5.9(2017):7700-7708.