The influence of air annealing on the microstructure and scintillation properties of Ce,Mg:LuAG ceramics | |
Chen, Xiaopu1,2; Hu, Zewang1,2; Dai, Jiawei1,2; Chen, Haohong1; Shi, Yun1; Kou, Huamin1; Wang, Tiantian2; Vedda, Anna3; Beitlerova, Alena4; Kucerkova, Romana4 | |
刊名 | Journal of the American Ceramic Society
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2018 | |
ISSN号 | 00027820 |
DOI | 10.1111/jace.16038 |
英文摘要 | The microstructures and optical properties of Ce,Mg:Lu3Al5O12 scintillator ceramics are investigated with particular focus on the effect of postannealing in air from 1000 to 1450°C. The formation of Al2O3 clusters after annealing above 1300°C is evidenced by scanning electron microscopy. The presence of this secondary phase is tentatively explained by the occurrence of Ce and Mg evaporation, proved by inductive coupled plasma optical emission spectrometry measurements, followed by defect diffusion and clustering during high temperature annealing. Meanwhile, optical investigations including absorption, X-ray induced luminescence, light yield, scintillation decay, and thermoluminescence prove the positive role of post-annealing that leads to a brighter and faster scintillation emission. This behavior is associated to the removal of oxygen vacancies occurring during such treatments. In parallel, the partial conversion of Ce3+ ions into Ce4+ is also observed as a consequence of annealings and the role of Ce4+ ions in the scintillation process is discussed. © 2018 The American Ceramic Society |
出版者 | Blackwell Publishing Inc. |
内容类型 | 期刊论文 |
源URL | [http://ir.sic.ac.cn/handle/331005/25343] ![]() |
专题 | 中国科学院上海硅酸盐研究所 |
作者单位 | 1.Key Laboratory of Transparent Opto-functional Inorganic Materials, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, China; 2.University of Chinese Academy of Sciences, Beijing, China; 3.Department of Materials Science, University of Milano-Bicocca, Milano, Italy; 4.Institute of Physics, Academy of Sciences of the Czech Republic, Prague, Czech Republic |
推荐引用方式 GB/T 7714 | Chen, Xiaopu,Hu, Zewang,Dai, Jiawei,et al. The influence of air annealing on the microstructure and scintillation properties of Ce,Mg:LuAG ceramics[J]. Journal of the American Ceramic Society,2018. |
APA | Chen, Xiaopu.,Hu, Zewang.,Dai, Jiawei.,Chen, Haohong.,Shi, Yun.,...&Li, Jiang.(2018).The influence of air annealing on the microstructure and scintillation properties of Ce,Mg:LuAG ceramics.Journal of the American Ceramic Society. |
MLA | Chen, Xiaopu,et al."The influence of air annealing on the microstructure and scintillation properties of Ce,Mg:LuAG ceramics".Journal of the American Ceramic Society (2018). |
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