Design Synthesis of ITE Zeolite Using Nickel-Amine Complex as an Efficient Structure-Directing Agent

doi:10.1021/acsami.8b10620

CORC > 武汉物理与数学研究所 > 中国科学院武汉物理与数学研究所 > 磁共振应用研究部

	Design Synthesis of ITE Zeolite Using Nickel-Amine Complex as an Efficient Structure-Directing Agent
	Xiao, Feng-Shou 4; Meng, Xiangju 4; Jin, Chuanhong 1; Zheng, Anmin 2; Zhu, Longfeng 3,4; Wang, Liang 4; Zhang, Jian 4; Chen, Wei 2; Wu, Qinming 1,4; Han, Shichao 4
刊名	ACS APPLIED MATERIALS & INTERFACES
	2018-10-03
卷号	10 期号:39 页码:33214-33220
关键词	zeolite ITE nickel-pentaethylenexamine design synthesis hydrogenation of CO2
ISSN号	1944-8244
DOI	10.1021/acsami.8b10620
英文摘要	Modern methodologies for synthesizing zeolites typically involve the employment of costly organic structure-directing agents. Herein, we report the design synthesis of aluminosilicate zeolite with ITE structure using an inexpensive nickel amine complex (nickel-pentaethylenexamine) as a novel structure-directing agent. Characterizations including X-ray diffraction, scanning electron microscopy, N-2 sorption isotherms, and Al-27 magic-angle spinning NMR techniques show that the ITE zeolite has high crystallinity, perfect crystals, large surface area, and abundant aluminum species in the framework. More importantly, catalytic tests on the hydrogenation of CO2 into methane show that the Ni-ITE zeolite exhibits better catalytic performance than aluminosilicate-supported and silica-supported nickel catalysts. Obviously, the use of nickel amine complex offers an alternative and facile way to synthesize aluminosilicate zeolites.
资助项目	National Key Research and Development Program of China[2017YFB0702803] ; National Natural Science Foundation of China[91634201] ; National Natural Science Foundation of China[91545111] ; National Natural Science Foundation of China[21703203] ; National Natural Science Foundation of China[21802053] ; National Natural Science Foundation of China[21720102001] ; China Postdoctoral Science Foundation[2017M611978]
WOS关键词	SELECTIVE CATALYTIC-REDUCTION ; CARBON-DIOXIDE METHANATION ; ONE-POT SYNTHESIS ; CRYSTAL-STRUCTURE ; ACTIVE CATALYST ; FRAMEWORK ; TEMPLATE ; SILICA ; NANOPARTICLES ; STA-7
WOS研究方向	Science & Technology - Other Topics ; Materials Science
语种	英语
出版者	AMER CHEMICAL SOC
WOS记录号	WOS:000446919800031
资助机构	National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation
内容类型	期刊论文
源URL	[http://ir.wipm.ac.cn/handle/112942/13305]
专题	武汉物理与数学研究所_磁共振应用研究部
通讯作者	Meng, Xiangju; Wu, Qinming
作者单位	1.Zhejiang Univ, Sch Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310007, Zhejiang, Peoples R China 2.Wuhan Inst Phys & Math, Wuhan Ctr Magnet Resonance, State Key Lab Magnet Resonance & Atom & Mol Phys, Wuhan 430071, Hubei, Peoples R China 3.Jiaxing Univ, Coll Biol Chem Sci & Engn, Jiaxing 314001, Peoples R China 4.Zhejiang Univ, Key Lab Appl Chem Zhejiang Prov, Hangzhou 310028, Zhejiang, Peoples R China
推荐引用方式 GB/T 7714	Xiao, Feng-Shou,Meng, Xiangju,Jin, Chuanhong,et al. Design Synthesis of ITE Zeolite Using Nickel-Amine Complex as an Efficient Structure-Directing Agent[J]. ACS APPLIED MATERIALS & INTERFACES,2018,10(39):33214-33220.
APA	Xiao, Feng-Shou.,Meng, Xiangju.,Jin, Chuanhong.,Zheng, Anmin.,Zhu, Longfeng.,...&Han, Shichao.(2018).Design Synthesis of ITE Zeolite Using Nickel-Amine Complex as an Efficient Structure-Directing Agent.ACS APPLIED MATERIALS & INTERFACES,10(39),33214-33220.
MLA	Xiao, Feng-Shou,et al."Design Synthesis of ITE Zeolite Using Nickel-Amine Complex as an Efficient Structure-Directing Agent".ACS APPLIED MATERIALS & INTERFACES 10.39(2018):33214-33220.