Glucose production from lignocellulosic biomass using a membrane-based polymeric solid acid catalyst | |
Qi, Benkun1,2; Anh Vu1; Wickramasinghe, S. Ranil1; Qian, Xianghong3 | |
刊名 | BIOMASS & BIOENERGY |
2018-10-01 | |
卷号 | 117页码:137-145 |
关键词 | Biomass Cellulose Glucose Solid Acid Catalyst Membrane |
ISSN号 | 0961-9534 |
DOI | 10.1016/j.biombioe.2018.07.017 |
英文摘要 | Large-scale production of biomass-derived fuels and chemicals requires the economical and efficient depolymerization of lignocellulosic biomass into sugars and fuels. Catalytic hydrolysis of raw wheat straw for the production of glucose was conducted using a designed porous membrane-based polymeric solid acid catalyst consisting of poly (ionic liquid) and polysulfonic acid chains. The catalyst demonstrated superior activity and selectivity with glucose yield reached over 50% from the un-pretreated raw straw. Under the optimal conditions, over 80% of cellulose and over 90% of xylan were converted to soluble sugars and furans with over 60% glucose or xylose yields reached respectively from pretreated straw biomass. Our catalyst demonstrates high glucose and total reducing sugar (TRS) yields from lignocellulosic biomass with promising application for the future lignocellulosic biorefinery. |
资助项目 | NSF[CBET 1264896] ; Chinese Scholarship Council[201604910231] |
WOS关键词 | Molecular-dynamics Simulations ; Free-energy Landscape ; Cellulose-i-beta ; Ionic Liquids ; Condensation-reactions ; Gamma-valerolactone ; Aqueous-solution ; Rice Straw ; Hydrolysis ; Saccharification |
WOS研究方向 | Agriculture ; Biotechnology & Applied Microbiology ; Energy & Fuels |
语种 | 英语 |
出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
WOS记录号 | WOS:000442603700017 |
资助机构 | NSF ; Chinese Scholarship Council |
内容类型 | 期刊论文 |
源URL | [http://ir.ipe.ac.cn/handle/122111/25896] |
专题 | 中国科学院过程工程研究所 |
通讯作者 | Qian, Xianghong |
作者单位 | 1.Univ Arkansas, Ralph E Martin Dept Chem Engn, Fayetteville, AR 72701 USA 2.Univ Chinese Acad Sci, Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China 3.Univ Arkansas, Dept Biomed Engn, Fayetteville, AR 72701 USA |
推荐引用方式 GB/T 7714 | Qi, Benkun,Anh Vu,Wickramasinghe, S. Ranil,et al. Glucose production from lignocellulosic biomass using a membrane-based polymeric solid acid catalyst[J]. BIOMASS & BIOENERGY,2018,117:137-145. |
APA | Qi, Benkun,Anh Vu,Wickramasinghe, S. Ranil,&Qian, Xianghong.(2018).Glucose production from lignocellulosic biomass using a membrane-based polymeric solid acid catalyst.BIOMASS & BIOENERGY,117,137-145. |
MLA | Qi, Benkun,et al."Glucose production from lignocellulosic biomass using a membrane-based polymeric solid acid catalyst".BIOMASS & BIOENERGY 117(2018):137-145. |
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