Characterization of Gas-Phase Organics Using Proton Transfer Reaction Time-of-Flight Mass Spectrometry: Residential Coal Combustion

doi:10.1021/acs.est.7b03960

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	Characterization of Gas-Phase Organics Using Proton Transfer Reaction Time-of-Flight Mass Spectrometry: Residential Coal Combustion
	Cao, Junji 2; Baltensperger, Urs 3; Slowik, Jay G.3; El Haddad, Imad 3; Marchand, Nicolas 1; Kilic, Dogushan 3; Pospisilova, Veronika 3; Temime-Roussel, Brice 1; Bertrand, Amelie 1; Ni, Haiyan 2
刊名	ENVIRONMENTAL SCIENCE & TECHNOLOGY
	2018-03-06
卷号	52 期号:5 页码:2612-2617
DOI	10.1021/acs.est.7b03960
文献子类	Article
英文摘要	Residential coal combustion is a significant contributor to particulate urban air pollution in Chinese mega cities and some regions in Europe. While the particulate emission factors and the chemical characteristics of the organic and inorganic aerosol from coal combustion have been extensively studied, the chemical composition and nonmethane organic gas (NMOG) emission factors from residential coal combustion are mostly unknown. We conducted 23 individual burns in a traditional Chinese stove used for heating and cooking using five different coals with Chinese origins, characterizing the NMOG emissions using a proton transfer reaction time-of-flight mass spectrometer. The measured emission factors range from 1.5 to 14.1 g/kg(coal) for bituminous coals and are below 0.1 g/kg(coal) A for anthracite coals. The emission factors from the bituminous coals are mostly influenced by the time until the coal is fully ignited. The emissions from the bituminous coals are dominated by aromatic and oxygenated aromatic compounds with a significant contribution of hydrocarbons. The results of this study can help to improve urban air pollution modeling in China and Eastern Europe and can be used to constrain a coal burning factor in ambient gas phase positive matrix factorization studies.
WOS关键词	HOUSEHOLD STOVES ; EMISSION FACTORS ; WOOD COMBUSTION ; HAZE EVENTS ; CHINA ; COOKSTOVES ; ATMOSPHERE ; POLLUTION ; CARBON ; PM2.5
WOS研究方向	Engineering ; Environmental Sciences & Ecology
语种	英语
WOS记录号	WOS:000427202700023
内容类型	期刊论文
源URL	[http://ir.ieecas.cn/handle/361006/5226]
专题	地球环境研究所_粉尘与环境研究室
作者单位	1.Aix Marseille Univ, CNRS, LCE, F-13331 Marseille, France 2.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Key Lab Aerosol Chem & Phys, Xian 710061, Shaanxi, Peoples R China 3.Paul Scherrer Inst, Lab Atmospher Chem, CH-5232 Villigen, Switzerland
推荐引用方式 GB/T 7714	Cao, Junji,Baltensperger, Urs,Slowik, Jay G.,et al. Characterization of Gas-Phase Organics Using Proton Transfer Reaction Time-of-Flight Mass Spectrometry: Residential Coal Combustion[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2018,52(5):2612-2617.
APA	Cao, Junji.,Baltensperger, Urs.,Slowik, Jay G..,El Haddad, Imad.,Marchand, Nicolas.,...&Huang, Ru-Jin.(2018).Characterization of Gas-Phase Organics Using Proton Transfer Reaction Time-of-Flight Mass Spectrometry: Residential Coal Combustion.ENVIRONMENTAL SCIENCE & TECHNOLOGY,52(5),2612-2617.
MLA	Cao, Junji,et al."Characterization of Gas-Phase Organics Using Proton Transfer Reaction Time-of-Flight Mass Spectrometry: Residential Coal Combustion".ENVIRONMENTAL SCIENCE & TECHNOLOGY 52.5(2018):2612-2617.