Different dye removal mechanisms between monodispersed and uniform hexagonal thin plate-like MgAl-CO32--LDH and its calcined product in efficient removal of Congo red from water | |
Li, Bing1; Zhang, Yongxing1; Zhou, Xiangbo1; Liu, Zhongliang1; Liu, Qinzhuang1; Li, Xuanhua2,3 | |
刊名 | JOURNAL OF ALLOYS AND COMPOUNDS |
2016-07-15 | |
卷号 | 673期号:无页码:265-271 |
关键词 | Ldh Thin Plate-like Adsorption Mechanisms Organic Pollutants Adsorption |
DOI | 10.1016/j.jallcom.2016.02.248 |
文献子类 | Article |
英文摘要 | Monodispersed and uniform hexagonal thin plate-like magnesium-aluminum layered double hydroxide intercalated with CO32- (MgAl-CO32--LDH) is synthesized by an ethanol-water mediated solvothermal method. The maximum adsorption capacities of the as-synthesized and calcined MgAl - CO32- - LDH are 129.9 and 143.27 mg g(-1), respectively, which are higher than those of the other metal oxide nano-structures reported to date. More importantly, although N-2 adsorption-desorption analysis indicates that the BET surface area changed from 24.74 m(2) g(-1) for the as-synthesized MgAl - CO32- - LDH to 165.07 m(2) g(-1) for the calcined MgAl - CO32- - LDH, the as-synthesized and calcined hexagonal thin plate-like MgAl - CO32- - LDH structures show similar adsorption capacity of Congo red (CR) from aqueous solution. The adsorption mechanism for the as-prepared LDH is anion exchange while adsorption mechanism for the calcined LDH is reconstruction. Our study opens a new insight for understanding and preparing high-performance adsorbents for organic dye removal. (C) 2016 Elsevier B.V. All rights reserved. |
WOS关键词 | LAYERED DOUBLE HYDROXIDES ; SOLVOTHERMAL SYNTHESIS ; ADSORPTION PERFORMANCE ; ORGANIC POLLUTANTS ; HEAVY-METAL ; MG ; NANOSHEETS ; PHOTOCATALYSTS ; NANOSTRUCTURES ; NANOCRYSTALS |
WOS研究方向 | Chemistry ; Materials Science ; Metallurgy & Metallurgical Engineering |
语种 | 英语 |
WOS记录号 | WOS:000373466400035 |
资助机构 | National Natural Science Foundation of China(51302102 ; National Natural Science Foundation of China(51302102 ; National Natural Science Foundation of China(51302102 ; National Natural Science Foundation of China(51302102 ; National Natural Science Foundation of China(51302102 ; National Natural Science Foundation of China(51302102 ; National Natural Science Foundation of China(51302102 ; National Natural Science Foundation of China(51302102 ; Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Huaibei Scientific Talent Development Scheme(20130303 ; Huaibei Scientific Talent Development Scheme(20130303 ; Huaibei Scientific Talent Development Scheme(20130303 ; Huaibei Scientific Talent Development Scheme(20130303 ; Huaibei Scientific Talent Development Scheme(20130303 ; Huaibei Scientific Talent Development Scheme(20130303 ; Huaibei Scientific Talent Development Scheme(20130303 ; 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Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Foundation of Anhui Province(1408085QA19 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; Natural Science Research Project for Colleges and Universities of Anhui Province(KJ2016A638 ; 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内容类型 | 期刊论文 |
源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/22041] |
专题 | 合肥物质科学研究院_中科院固体物理研究所 |
作者单位 | 1.Huaibei Normal Univ, Collaborat Innovat Ctr Adv Funct Composites, Huibei 235000, Peoples R China 2.Northwestern Polytech Univ, Sch Mat Sci & Engn, State Key Lab Solidificat Proc, Ctr Nano Energy Mat, Xian 710072, Peoples R China 3.Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Peoples R China |
推荐引用方式 GB/T 7714 | Li, Bing,Zhang, Yongxing,Zhou, Xiangbo,et al. Different dye removal mechanisms between monodispersed and uniform hexagonal thin plate-like MgAl-CO32--LDH and its calcined product in efficient removal of Congo red from water[J]. JOURNAL OF ALLOYS AND COMPOUNDS,2016,673(无):265-271. |
APA | Li, Bing,Zhang, Yongxing,Zhou, Xiangbo,Liu, Zhongliang,Liu, Qinzhuang,&Li, Xuanhua.(2016).Different dye removal mechanisms between monodispersed and uniform hexagonal thin plate-like MgAl-CO32--LDH and its calcined product in efficient removal of Congo red from water.JOURNAL OF ALLOYS AND COMPOUNDS,673(无),265-271. |
MLA | Li, Bing,et al."Different dye removal mechanisms between monodispersed and uniform hexagonal thin plate-like MgAl-CO32--LDH and its calcined product in efficient removal of Congo red from water".JOURNAL OF ALLOYS AND COMPOUNDS 673.无(2016):265-271. |
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