Defect suppression in AlN epilayer using hierarchical growth units | |
Zhuang, Qi ; Lin, Wei ; Yang, Weihuang ; Yang, Wencao ; Huang, Chengcheng ; Li, Jinchai ; Chen, Hangyang ; Li, Shuping ; Kang, Junyong ; Chen HY(陈航洋) ; Kang JY(康俊勇) | |
刊名 | http://dx.doi.org/10.1021/jp401745v |
2013-07-11 | |
关键词 | Atomic force microscopy Defects Grain boundaries Luminescence Vapors |
英文摘要 | Growing AlN layers remains a significant challenge because it is subject to a large volume fraction of grain boundaries. In this study, the nature and formation of the AlN growth mechanism is examined by ab initio simulations and experimental demonstration. The calculated formation enthalpies of the constituent elements, including the Al/N atom, Al-N molecule, and Al-N 3 cluster, vary with growth conditions in N-rich and Al-rich environments. Using the calculation results as bases, we develop a three-step metalorganic vapor-phase epitaxy, which involves the periodic growth sequence of (i) trimethylaluminum (TMAl), (ii) ammonia (NH3), and (iii) TMAl+NH3 supply, bringing in hierarchical growth units to improve AlN layer compactness. A series of AlN samples were grown, and their morphological and luminescent evolutions were evaluated by atomic force microscopy and cathodoluminescence, respectively. The proposed technique is advantageous because the boundaries and defect-related luminescence derived are highly depressed, serving as a productive platform from which to further optimize the properties of AlGaN semiconductors. ? 2013 American Chemical Society. |
语种 | 英语 |
出版者 | American Chemical Society |
内容类型 | 期刊论文 |
源URL | [http://dspace.xmu.edu.cn/handle/2288/91958] |
专题 | 物理技术-已发表论文 |
推荐引用方式 GB/T 7714 | Zhuang, Qi,Lin, Wei,Yang, Weihuang,et al. Defect suppression in AlN epilayer using hierarchical growth units[J]. http://dx.doi.org/10.1021/jp401745v,2013. |
APA | Zhuang, Qi.,Lin, Wei.,Yang, Weihuang.,Yang, Wencao.,Huang, Chengcheng.,...&康俊勇.(2013).Defect suppression in AlN epilayer using hierarchical growth units.http://dx.doi.org/10.1021/jp401745v. |
MLA | Zhuang, Qi,et al."Defect suppression in AlN epilayer using hierarchical growth units".http://dx.doi.org/10.1021/jp401745v (2013). |
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