Effect of Pulse Shaping on Observing Coherent Energy Transfer in Single Light-Harvesting Complexes

CORC > 化学研究所 > 中国科学院化学研究所 > 分子动态与稳态结构实验室

	Effect of Pulse Shaping on Observing Coherent Energy Transfer in Single Light-Harvesting Complexes
	Song, Kai 1; Bai, Shuming 1,2; Shi, Qiang 1,2
刊名	JOURNAL OF PHYSICAL CHEMISTRY B
	2016-11-17
卷号	120 期号:45 页码:11637-11643
英文摘要	Recent experimental and theoretical studies have revealed that quantum coherence plays an important role in the excitation energy transfer in photosynthetic light harvesting (LH) complexes. Inspired by the recent single-molecule two-color double-pump experiment, we theoretically investigate the effect of pulse shaping on observing coherent energy transfer in the single bacterial LH2 complex. It is found that quantum coherent energy transfer can be observed when the time delay and phase difference between the two laser pulses are controlled independently. However, when the two-color pulses are generated using the pulse-shaping method, how the laser pulses are prepared is crucial to the observation of quantum coherent energy transfer in single photosynthetic complexes.
收录类别	SCI
语种	英语
内容类型	期刊论文
源URL	[http://ir.iccas.ac.cn/handle/121111/35723]
专题	化学研究所_分子动态与稳态结构实验室
作者单位	1.Chinese Acad Sci, Inst Chem, State Key Lab Struct Chem Unstable & Stable Speci, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式 GB/T 7714	Song, Kai,Bai, Shuming,Shi, Qiang. Effect of Pulse Shaping on Observing Coherent Energy Transfer in Single Light-Harvesting Complexes[J]. JOURNAL OF PHYSICAL CHEMISTRY B,2016,120(45):11637-11643.
APA	Song, Kai,Bai, Shuming,&Shi, Qiang.(2016).Effect of Pulse Shaping on Observing Coherent Energy Transfer in Single Light-Harvesting Complexes.JOURNAL OF PHYSICAL CHEMISTRY B,120(45),11637-11643.
MLA	Song, Kai,et al."Effect of Pulse Shaping on Observing Coherent Energy Transfer in Single Light-Harvesting Complexes".JOURNAL OF PHYSICAL CHEMISTRY B 120.45(2016):11637-11643.